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Register a new userEnhanced and directional single photon emission in hyperbolic metamaterials
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We propose an approach to enhance and direct the spontaneous emission from isolated emitters embedded inside hyperbolic metamaterials into single photon beams. The approach rests on collective plasmonic Bloch modes of hyperbolic metamaterials which propagate in highly directional beams called quantum resonance cones. We propose a pumping scheme using the transparency window of the hyperbolic metamaterial that occurs near the topological transition. Finally, we address the challenge of outcoupling these broadband resonance cones into vacuum using a dielectric bullseye grating. We give a detailed analysis of quenching and design the metamaterial to have a huge Purcell factor in a broad bandwidth inspite of the losses in the metal. Our work should help motivate experiments in the development of single photon sources for broadband emitters such as nitrogen vacancy centers in diamond.
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In this paper we reveal the physics behind the formation of tri- and tetra-hyperbolic phases in anisotropic metamaterials without magnetoelectric coupling and describe the anti-crossing splitting phenomenon in the hyperbolic dispersion which arises due to the hybridization of the plasmonic and magnetic Bloch high-k polaritons. This considerably deepens the understanding of the high-k polaritons and the topology of the optical iso-frequency surfaces in k-space and will find applications in optical nano-resolution imaging and emission rate and directivity control. To accomplish this, we develop a range of new techniques of theoretical optics for bianisotropic materials, including the quadratic index of refraction operator method, suitable to study the high-k polaritons with finite indices of refraction and the explicit expression for the characteristic matrix in generic bianisotropic media. We introduce the spatial stratification approach for the electric and magnetic responses of anisotropic homogeneous media to analyze the underlying Bloch waves. We believe that the formalisms developed here can be useful for the researchers in the field of theoretical optics of anisotropic and bianisotropic media in the future.
Hyperbolic Metamaterials (HMMs) have recently garnered much attention because they possess the ability for broadband manipulation of the photon density of states and sub-wavelength light confinement. However, a major difficulty arises with the coupling of light out of HMMs due to strong confinement of the electromagnetic field in states with high momentum called high-k modes which become evanescent outside the structure. Here we report the first demonstration of directional out-coupling of light from high-k modes in an active HMM using a high index bulls-eye grating. Quantum dots (QDs) embedded underneath the metamaterial show highly directional emission through the propagation and out-coupling of resonance cones which are a unique feature of hyperbolic media. This demonstration of efficient out-coupling of light from active HMMs could pave the way for developing practical photonic devices using these systems.
Sub-wavelength nanostructured systems with tunable electromagnetic properties, such as hyperbolic metamaterials (HMMs), provide a useful platform to tailor spontaneous emission processes. Here, we investigate a system comprising $Eu^{ 3+}(NO_{3})_{3}6H_{2}O$ nanocrystals on an HMM structure featuring a hexagonal array of Ag-nanowires in a porous $Al_{2}O_{3}$ matrix. The HMM-coupled $Eu^{ 3+}$ ions exhibit up to a 2.4-fold increase of their decay rate, accompanied by an enhancement of the emission rate of the $^{ 5}D_{0}rightarrow$ $^{ 7}F_{2}$ transition. Using finite-difference time-domain modeling, we corroborate these observations with the increase in the photonic density of states seen by the $Eu^{ 3+}$ ions in the proximity of the HMM. Our results indicate HMMs can serve as a valuable tool to control the emission from weak transitions, and hence hint at a route towards more practical applications of rare-earth ions in nanoscale optoelectronics and quantum devices.
The optical properties of some nanomaterials can be controlled by an external magnetic field, providing active functionalities for a wide range of applications, from single-molecule sensing to nanoscale nonreciprocal optical isolation. Materials with broadband tunable magneto-optical response are therefore highly desired for various components in next-generation integrated photonic nanodevices. Concurrently, hyperbolic metamaterials received a lot of attention in the past decade since they exhibit unusual properties that are rarely observed in nature and provide an ideal platform to control the optical response at the nanoscale via careful design of the effective permittivity tensor, surpassing the possibilities of conventional systems. Here, we experimentally study magnetic circular dichroism in a metasurface made of type-II hyperbolic nanoparticles on a transparent substrate. Numerical simulations confirm the experimental findings, and an analytical model is established to explain the physical origin of the observed magneto-optical effects, which can be described in terms of the coupling of fundamental electric and magnetic dipole modes with an external magnetic field. Our system paves the way for the development of nanophotonic active devices combining the benefits of sub-wavelength light manipulation in hyperbolic metamaterials supporting a large density of optical states with the ability to freely tune the magneto-optical response via control over the anisotropic permittivity of the system.
Hyperbolic metamaterials (HMMs) support propagating waves with arbitrarily large wavevectors over broad spectral ranges, and are uniquely valuable for engineering radiative thermal transport in the near field. Here, by employing a rational design approach based on the electromagnetic local density of states, we demonstrate the ability of HMMs to substantially rectify radiative heat flow. Our idea is to establish a forward-biased scenario where the two HMM-based terminals of a thermal diode feature overlapped hyperbolic bands which result in a large heat current, and suppress the reverse heat flow by creating spectrally mismatched density of states as the temperature bias is flipped. As an example, we present a few high-performance thermal diodes by pairing HMMs made of polar dielectrics and metal-to-insulator transition (MIT) materials in the form of periodic nanowire arrays, and considering three representative kinds of substrates. Upon optimization, we theoretically achieve a rectification ratio of 324 at a 100 nm gap, which remains greater than 148 for larger gap sizes up to 1 um over a wide temperature range. The maximum rectification represents an almost 1000-fold increase compared to a bulk diode using the same materials, and is twice that of state-of-the-art designs. Our work highlights the potential of HMMs for rectifying radiative heat flow, and may find applications in advanced thermal management and energy conversion systems.
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