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Register a new userAlpha decay favoured isotopes of some superheavy nuclei: Spontaneous fission versus alpha decay
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Authors
O. V. Kiren
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Spontaneous fission and alpha decay are the main decay modes for superheavy nuclei. The superheavy nuclei which have small alpha decay half-life compared to spontaneous fission half-life will survive fission and can be detected in the laboratory through alpha decay. We have studied the alpha decay half-life and spontaneous half-life of some superheavy elements in the atomic range Z = 100-130. Spontaneous fission half-lives of superheavy nuclei have been calculated using the phenomenological formula and the alpha decay half-lives using Viola-Seaborg-Sobiczewski formula (Sobiczewski et al. 1989), semi empirical relation of Brown (1992) and formula based on generalized liquid drop model proposed by Dasgupta-Schubert and Reyes (2007). The results are reported here.
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Alpha-decay energies for several chains of super-heavy nuclei are calculated within the self-consistent mean-field approach by using the Fayans functional FaNDF$^0$. They are compared to the experimental data and predictions of two Skyrme functionals, SLy4 and SkM*, and of the macro-micro method as well. The corresponding lifetimes are calculated with the use of the semi-phenomenological formulas by Parkhomenko and Sobiczewski and by Royer and Zhang.
New recent experimental $alpha$ decay half-lives have been compared with the results obtained from previously proposed formulas depending only on the mass and charge numbers of the $alpha$ emitter and the Q$alpha$ value. For the heaviest nuclei they are also compared with calculations using the Density-Dependent M3Y (DDM3Y) effective interaction and the Viola-Seaborg-Sobiczewski (VSS) formulas. The correct agreement allows us to make predictions for the $alpha$ decay half-lives of other still unknown superheavy nuclei from these analytic formulas using the extrapolated Q$alpha$ of G. Audi, A. H. Wapstra, and C. Thibault [Nucl. Phys. A729, 337 (2003)].
Experimental $alpha$-decay half-life, spin, and parity of 398 nuclei in the range 50$leq$Z$leq$118 are utilized to propose a new formula (QF) with only 4 coefficients as well as to modify the Tagepera-Nurmia formula with just 3 coefficients (MTNF) by employing nonlinear regressions. These formulas, based on reduced mass ($mu$) and angular momentum taken away by the $alpha$-particle, are ascertained very effective for both favoured and unfavoured $alpha$-decay in addition to their excellent match with all (Z, N) combinations of experimental $alpha$-decay half-lives. After comparing with similar other empirical formulas of $alpha$-decay half-life, QF and MTNF formulas are purported with accuracy, minimum uncertainty and deviation, dependency on least number of fitted coefficients together with less sensitivity to the uncertainties of $Q$-values. The QF formula is applied to predict $alpha$-decay half-lives for 724 favoured and 635 unfavoured transitions having experimentally known $Q$-values. Moreover, these available $Q$-values are also employed to test various theoretical approaches viz. RMF, FRDM, WS4, RCHB, etc. along with machine learning method XGBoost for determining theoretical $Q$-values, incisively. Thereafter, using $Q$-values from the most precise theoretical treatment mentioned above along with the proposed formulas, probable $alpha$-decay chains for Z$=$120 isotopes are identified.
A quantum mechanical analysis of the bremsstrahlung in $alpha$ decay of $^{210}$Po is performed in close reference to a semiclassical theory. We clarify the contribution from the tunneling, mixed, outside barrier regions and from the wall of the inner potential well to the final spectral distribution, and discuss their interplay. We also comment on the validity of semiclassical calculations, and the possibility to eliminate the ambiguity in the nuclear potential between the alpha particle and daughter nucleus using the bremsstrahlung spectrum.
A recent high-resolution $alpha$, $X$-ray, and $gamma$-ray coincidence-spectroscopy experiment offered first glimpse of excitation schemes of isotopes along $alpha$-decay chains of $Z=115$. To understand these observations and to make predictions about shell structure of superheavy nuclei below $^{288}115$, we employ two complementary mean-field models: self-consistent Skyrme Energy Density Functional approach and the macroscopic-microscopic Nilsson model. We discuss the spectroscopic information carried by the new data. In particular, candidates for the experimentally observed $E1$ transitions in $^{276}$Mt are proposed. We find that the presence and nature of low-energy $E1$ transitions in well-deformed nuclei around $Z=110, N=168$ strongly depends on the strength of the spin-orbit coupling; hence, it provides an excellent constraint on theoretical models of superheavy nuclei. To clarify competing theoretical scenarios, an experimental search for $E1$ transitions in odd-$A$ systems $^{275,277}$Mt, $^{275}$Hs, and $^{277}$Ds is strongly recommended.
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