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Register a new userBrillouin Light Scattering Spectra as local Temperature Sensors for Thermal Magnons and Acoustic Phonons
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We demonstrate the use of the micro-Brillouin light scattering (micro-BLS) technique as a local temperature sensor for magnons in a Permalloy thin film and phonons in the glass substrate. A systematic shift in the frequencies of two thermally excited perpendicular standing spin wave modes as the film is uniformly heated allows us to achieve a temperature resolution better than 2.5 K. We demonstrate that the micro-BLS spectra can be used to measure the local temperatures of phonons and magnons across a thermal gradient. Such local temperature sensors are useful for investigating spin caloritronic and thermal transport phenomena in general.
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We report results of an investigation of the temperature dependence of the magnon and phonon frequencies in NiO. A combination of Brillouin - Mandelstam and Raman spectroscopies allowed us to elucidate the evolution of the phonon and magnon spectral signatures from the Brillouin zone center (GHz range) to the second-order peaks from the zone boundary (THz range). The temperature-dependent behavior of the magnon and phonon bands in the NiO spectrum indicates the presence of antiferromagnetic (AF) order fluctuation or a persistent AF state at temperatures above the Neel temperature (T=523 K). Tuning the intensity of the excitation laser provides a method for disentangling the features of magnons from acoustic phonons without the application of a magnetic field. Our results are useful for interpretation of the inelastic-light scattering spectrum of NiO, and add to the knowledge of its magnon properties important for THz spintronic devices.
The spectral distribution of parametrically excited dipole-exchange magnons in an in-plane magnetized epitaxial film of yttrium-iron garnet was studied by means of frequency- and wavevector-resolved Brillouin light scattering spectroscopy. The experiment was performed in a parallel pumping geometry where an exciting microwave magnetic field was parallel to the magnetizing field. It was found that for both dipolar and exchange spectral areas parallel pumping excites the lowest volume magnon modes propagating in the film plane perpendicularly to the magnetization direction. In order to interpret the experimental observations, we used a microscopic Heisenberg model that includes exchange as well as dipole-dipole interactions to calculate the magnon spectrum and construct the eigenstates. As proven in our calculations, the observed magnons are characterized by having the highest possible ellipticity of precession which suggests the lowest threshold of parametric generation. Applying different pumping powers we observe modifications in the magnon spectrum that are described theoretically by a softening of the spin stiffness.
The phonon density of states (DOS) and magnetic excitation spectrum of polycrystalline BiFeO$_3$ were measured for temperatures $200 leq T leq 750,$K, using inelastic neutron scattering (INS). Our results indicate that the magnetic spectrum of BiFeO$_3$ closely resembles that of similar Fe perovskites, such as LaFeO$_3$, despite the cycloid modulation in BiFeO$_3$. We do not find any evidence for a spin gap. A strong $T$-dependence of the phonon DOS was found, with a marked broadening of the whole spectrum, providing evidence of strong anharmonicity. This anharmonicity is corroborated by large-amplitude motions of Bi and O ions observed with neutron diffraction. These results highlight the importance of spin-phonon coupling in this material.
Brillouin light scattering in ferromagnetic materials usually involves one magnon and two photons and their total angular momentum is conserved. Here, we experimentally demonstrate the presence of a helicity-changing two-magnon Brillouin light scattering in a ferromagetic crystal, which can be viewed as a four-wave mixing process involving two magnons and two photons. Moreover, we observe an unconventional helicity-changing one-magnon Brillouin light scattering, which apparently infringes the conservation law of the angular momentum. We show that the crystal angular momentum intervenes to compensate the missing angular momentum in the latter scattering process.
Magnons are the energy quanta of fundamental spin excitations, namely spin waves, and they can make a considerable contribution to energy transport in some magnetic materials in a similar manner as lattice vibration waves or phonons. The coupling and possible non-equilibrium between magnons and other energy carriers have been used to explain several recently discovered thermally driven spin transport and energy conversion phenomena. Here, we report experiments in which local non-equilibrium between magnons and phonons in a single crystalline bulk magnetic insulator, Y3Fe5O12 (yttrium iron garnet, or YIG), has been created optically within a focused laser spot and probed directly with the use of micro-Brillouin light scattering (BLS). By analyzing the experimental results with a thermally induced magnon diffusion model, we obtain the magnon diffusion length of thermal magnons. By explicitly establishing non-equilibrium between magnons and phonons, our studies represent an important step toward a quantitative understanding of various spin-heat coupling phenomena.
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