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Register a new userRandom quasi-phase-matched second-harmonic generation in periodically poled lithium tantalate
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Added by
Alessandro Busacca C.
Publication date
2012
fields
Physics
and research's language is
English
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We observe second harmonic generation via random quasi-phase-matching in a 2.0 mu m periodically poled, 1-cm-long, z-cut lithium tantalate. Away from resonance, the harmonic output profiles exhibit a characteristic pattern stemming from a stochastic domain distribution and a quadratic growth with the fundamental excitation, as well as a broadband spectral response. The results are in good agreement with a simple model and numerical simulations in the undepleted regime, assuming an anisotropic spread of the random nonlinear component.
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Prospective integrated quantum optical technologies will combine nonlinear optics and components requiring cryogenic operating temperatures. Despite the prevalence of integrated platforms exploiting $chi^{(2)}$-nonlinearities for quantum optics, for example used for quantum state generation and frequency conversion, their material properties at low temperatures are largely unstudied. Here, we demonstrate the first second harmonic generation in a fiber-coupled lithium niobate waveguide at temperatures down to 4.4K. We observe a reproducible shift in the phase-matched pump wavelength within the telecom band, in addition to transient discontinuities while temperature cycling. Our results establish lithium niobate as a versatile nonlinear photonic integration platform compatible with cryogenic quantum technologies.
Optical waveguides made from periodically poled materials provide high confinement of light and enable the generation of new wavelengths via quasi-phase-matching, making them a key platform for nonlinear optics and photonics. However, such devices are not typically employed for high-harmonic generation. Here, using 200-fs, 10-nJ-level pulses of 4100 nm light at 1 MHz, we generate high harmonics up to the 13th harmonic (315 nm) in a chirped, periodically poled lithium niobate (PPLN) waveguide. Total conversion efficiencies into the visible--ultraviolet region are as high as 10 percent. We find that the output spectrum depends on the waveguide poling period, indicating that quasi-phase-matching plays a significant role. In the future, such periodically poled waveguides may enable compact sources of ultrashort pulses at high repetition rates and provide new methods of probing the electronic structure of solid-state materials.
Lithium niobate (LN), dubbed by many as the silicon of photonics, has recently risen to the forefront of chip-scale nonlinear optics research since its demonstration as an ultralow-loss integrated photonics platform. Due to its significant quadratic nonlinearity ($chi^{(2)}$), LN inspires many important applications such as second-harmonic generation (SHG), spontaneous parametric down-conversion, and optical parametric oscillation. Here, we demonstrate high-efficiency SHG in dual-resonant, periodically poled z-cut LN microrings, where quasi-phase matching is realized by field-assisted domain engineering. Meanwhile, dual-band operation is accessed by optimizing the coupling conditions in fundamental and second-harmonic bands via a single pulley waveguide. As a result, when pumping a periodically poled LN microring in the low power regime at around 1617nm, an on-chip SHG efficiency of 250,000%/W is achieved, a state-of-the-art value reported among current integrated photonics platforms. An absolute conversion efficiency of 15% is recorded with a low pump power of 115$mu$W in the waveguide. Such periodically poled LN microrings also present a versatile platform for other cavity-enhanced quasi-phase matched $chi^{(2)}$ nonlinear optical processes.
We demonstrate photon-pair generation in a reverse proton exchanged waveguide fabricated on a periodically poled magnesium doped stoichiometric lithium tantalate substrate. Detected pairs are generated via a cascaded second order nonlinear process where a pump laser at wavelength of 1.55 $mu$m is first doubled in frequency by second harmonic generation and subsequently downconverted around the same spectral region. Pairs are detected at a rate of 42 per second with a coincidence to accidental ratio of 0.7. This cascaded pair generation process is similar to four-wave-mixing where two pump photons annihilate and create a correlated photon pair.
Supercontinuum generation in integrated photonic waveguides is a versatile source of broadband light, and the generated spectrum is largely determined by the phase-matching conditions. Here we show that quasi-phase-matching via periodic modulations of the waveguide structure provides a useful mechanism to control the evolution of ultrafast pulses and the supercontinuum spectrum. We experimentally demonstrate quasi-phase-matched supercontinuum to the TE20 and TE00 waveguide modes, which enhances the intensity of the SCG in specific spectral regions by as much as 20 dB. We utilize higher-order quasi-phase-matching (up to the 16th order) to enhance the intensity in numerous locations across the spectrum. Quasi-phase-matching adds a unique dimension to the design-space for SCG waveguides, allowing the spectrum to be engineered for specific applications.
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