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Register a new userInelastic electron and Raman scattering from the collective excitations in quantum wires: Zero magnetic field
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Authors
Manvir S. Kushwaha
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The nanofabrication technology has taught us that an $m$-dimensional confining potential imposed upon an $n$-dimensional electron gas paves the way to a quasi-($n-m$)-dimensional electron gas, with $m le n$ and $1le n, m le 3$. This is the road to the (semiconducting) quasi-$n$ dimensional electron gas systems we have been happily traversing on now for almost three decades. Achieving quasi-one dimensional electron gas (Q-1DEG) [or quantum wire(s) for more practical purposes] led us to some mixed moments in this journey: while the reduced phase space for the scattering led us believe in the route to the faster electron devices, the proximity to the 1D systems left us in the dilemma of describing it as a Fermi liquid or as a Luttinger liquid. No one had ever suspected the potential of the former, but it took quite a while for some to convince the others on the latter. A realistic Q-1DEG system at the low temperatures is best describable as a Fermi liquid rather than as a Luttinger liquid. In the language of condensed matter physics, a critical scrutiny of Q-1DEG systems has provided us with a host of exotic (electronic, optical, and transport) phenomena revealing their unparallel behavior characteristics unseen in their higher or lower dimensional counterparts. Here, we embark on the systematic investigation of the inelastic electron scattering (IES) and of inelastic light scattering (ILS) from the elementary electronic excitations in quantum wires in the absence of an applied magnetic field. To that end, we begin with the Kubos correlation functions to derive the generalized nonlocal, dynamic dielectric function, the inverse dielectric function, and the Dyson equation for the dynamic screened potential in the framework of Bohm-Pines full and famous random-phase approximation...
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The most fundamental approach to an understanding of electronic, optical, and transport phenomena which the condensed matter physics (of conventional as well as nonconventional systems) offers is generally founded on two experiments: the inelastic electron scattering and the inelastic light scattering. This work embarks on providing a systematic framework for the theory of inelastic electron scattering and of inelastic light scattering from the electronic excitations in GaAs/Ga$_{1-x}$Al$_{x}$As quantum wells. To this end, we start with the Kubos correlation function to derive the generalized nonlocal, dynamic dielectric function, and the inverse dielectric function within the framework of Bohm-Pines random-phase approximation. This is followed by a thorough development of the theory of inelastic electron scattering and of inelastic light scattering. The methodological part is then subjected to the analytical diagnoses which allow us to sense the subtlety of the analytical results and the importance of their applications. The general analytical results, which know no bounds regarding, e.g., the subband occupancy, are then specified so as to make them applicable to practicality. After trying and testing the eigenfunctions, we compute the density of states, the Fermi energy, the full excitation spectrum made up of intrasubband and intersubband -- single-particle and collective (plasmon) -- excitations, the loss functions for all the principal geometries envisioned for the inelastic electron scattering, and the Raman intensity, which provides a measure of the real transitions induced by the (laser) probe, for the inelastic light scattering...
A theoretical investigation has been made of the magnetoplasmon excitations in a quasi-one-dimensional electron system comprised of vertically stacked, self-assembled InAs/GaAs quantum dots. The smaller length scales involved in the experiments impel us to consider a perfectly periodic system of two-dimensionally confined InAs quantum dot layers separated by GaAs spacers. Subsequent system is subjected to a two-dimensional confining (harmonic) potential in the x-y plane and an applied magnetic field (B) in the symmetric gauge. This scheme defines virtually a system of quantum wire comprised of vertically stacked quantum dots (VSQD). We derive and discuss the Dyson equation, the generalized (nonlocal and dynamic) dielectric function, and the inverse dielectric function for investigating the single-particle and collective (magnetoplasmon) excitations within the framework of (full) random-phase approximation (RPA). As an application, we study the influence of the confinement potential and the magnetic field on the component eigenfunctions, the density of states (DOS), the Fermi energy, the collective excitations, and the inverse dielectric functions. These findings demonstrate, for the very first time, the significance of investigating the system of VSQD subjected to a quantizing magnetic field. Given the edge over the planar quantum dots and the foreseen applications in the single-electron devices and quantum computation, investigating the system of VSQD is deemed vital. The results suggest exploiting magnetoplasmon qubits to be a potential option for implementing the solemn idea of quantum state transfer in devising quantum gates for the quantum computation and quantum communication networks.
Electron Raman scattering (ERS) is investigated in a parabolic semiconductor quantum wire in a transverse magnetic field neglecting by phonon-assisted transitions. The ERS cross-section is calculated as a function of a frequency shift and magnetic field. The process involves an interband electronic transition and an intraband transition between quantized subbands. We analyze the differential cross-section for different scattering configurations. We study selection rules for the processes. Some singularities in the Raman spectra are found and interpreted. The scattering spectrum shows density-of-states peaks and interband matrix elements maximums and a strong resonance when scattered frequency equals to the hybrid frequency or confinement frequency depending on the light polarization. Numerical results are presented for a GaAs/AlGaAs quantum wire.
We predict inelastic light scattering spectra from electron collective excitations in a coaxial quantum well embedded in a core-multishell GaAs/AlGaAs nanowire. The complex composition, the hexagonal cross section and the remote doping of typical samples are explicitly included, and the free electron gas is obtained by a DFT approach. Inelastic light scattering cross sections due to charge and spin collective excitations belonging to quasi-1D and quasi-2D states, which coexist in such radial heterostructures, are predicted in the non-resonant approximation from a fully three-dimensional multi-subband TDDFT formalism. We show that collective excitations can be classified in azimuthal, radial and longitudinal excitations, according to the associated density fluctuations, and we suggest that their character can be exposed by specific spectral dispersion of inelastic light scattering along different planes of the heterostructure.
Undoped GaAs/AlGaAs heterostructures have been used to fabricate quantum wires in which the average impurity separation is greater than the device size. We compare the behavior of the Zero-Bias Anomaly against predictions from Kondo and spin polarization models. Both theories display shortcomings, the most dramatic of which are the linear electron-density dependence of the Zero-Bias Anomaly spin-splitting at fixed magnetic field B and the suppression of the Zeeman effect at pinch-off.
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