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Register a new userEjection of quasi-free electron pairs from the helium atom ground state by single photon absorption
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Added by
Markus Sch\\\"offler S.
Publication date
2012
fields
Physics
and research's language is
English
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We investigate single photon double ionization (PDI) of helium at photon energies of 440 and 800 eV. We observe doubly charged ions with close to zero momentum corresponding to electrons emitted back-to-back with equal energy. These slow ions are the unique fingerprint of an elusive quasi-free PDI mechanism predicted by Amusia et al. nearly four decades years ago [J. Phys. B 8, 1248, (1975)] . It results from the non-dipole part of the electromagnetic interaction. Our experimental data are in excellent agreement with calculations performed using the convergent close coupling and time dependent close coupling methods.
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Phase-shift differences and amplitude ratios of the outgoing $s$ and $d$ continuum wave packets generated by two-photon ionization of helium atoms are determined from the photoelectron angular distributions obtained using velocity map imaging. Helium atoms are ionized with ultrashort extreme-ultraviolet free-electron laser pulses with a photon energy of 20.3, 21.3, 23.0, and 24.3 eV, produced by the SPring-8 Compact SASE Source test accelerator. The measured values of the phase-shift differences are distinct from scattering phase-shift differences when the photon energy is tuned to an excited level or Rydberg manifold. The difference stems from the competition between resonant and non-resonant paths in two-photon ionization by ultrashort pulses. Since the competition can be controlled in principle by the pulse shape, the present results illustrate a new way to tailor the continuum wave packet.
We propose to couple single atomic qubits to photons incident on a cavity containing an atomic ensemble of a different species that mediates the coupling via Rydberg interactions. Subject to a classical field and the cavity field, the ensemble forms a collective dark state which is resonant with the input photon, while excitation of a qubit atom leads to a secondary dark state that splits the cavity resonance. The two different dark state mechanisms yield zero and $pi$ reflection phase shifts and can be used to implement quantum gates between atomic and optical qubits.
We employ two-photon spectroscopy to study the vibrational states of the triplet ground state potential ($a^3Sigma^+$) of the $^{23}$Na$^{6}$Li molecule. Pairs of Na and Li atoms in an ultracold mixture are photoassociated into an excited triplet molecular state, which in turn is coupled to vibrational states of the triplet ground potential. Vibrational state binding energies, line strengths, and potential fitting parameters for the triplet ground $a^3Sigma^+$ potential are reported. We also observe rotational splitting in the lowest vibrational state.
The ground-state energies of one-electron homonuclear quasi-molecules for the nuclear charge number in the range Z=1-100 at the chemical distances R= 2/Z (in a.u.) are calculated. The calculations are performed for both point- and extended-charge nucleus cases using the Dirac-Fock-Sturm approach with the basis functions constructed from the one-center Dirac-Sturm orbitals. The critical distances R_cr, at which the ground-state level reaches the edge of the negative-energy Dirac continuum, are calculated for homonuclear quasi-molecules in the range: Z=85-100. It is found that in case of U_2^{183+} the critical distance R_cr = 38.42 fm for the point-charge nuclei and R_cr = 34.72 fm for extended nuclei.
Quantum blockade and entanglement play important roles in quantum information and quantum communication as quantum blockade is an effective mechanism to generate single photons (phonons) and entanglement is a crucial resource for quantum information processing. In this work, we propose a method to generate single entangled photon-phonon pairs in a hybrid optomechanical system. We show that photon blockade, phonon blockade, and photon-phonon correlation and entanglement can be observed via the atom-photon-phonon (tripartite) interaction, under the resonant atomic driving. The correlated and entangled single photons and single phonons, i.e., single entangled photon-phonon pairs, can be generated in both the weak and strong tripartite interaction regimes. Our results may have important applications in the development of highly complex quantum networks.
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