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Register a new userSynthetic partial waves in ultracold atomic collisions
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Interactions between particles can be strongly altered by their environment. We demonstrate a technique for modifying interactions between ultracold atoms by dressing the bare atomic states with light, creating an effective interaction of vastly increased range that scatters states of finite relative angular momentum at collision energies where only s-wave scattering would normally be expected. We collided two optically dressed neutral atomic Bose-Einstein condensates with equal, and opposite, momenta and observed that the usual s-wave distribution of scattered atoms was altered by the appearance of d- and g-wave contributions. This technique is expected to enable quantum simulation of exotic systems, including those predicted to support Majorana fermions.
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Helium atoms in the metastable $2^3{S_{1}}$ state (He$^*$) have unique advantages for ultracold atomic experiments. However, there is no known accessible Feshbach resonance in He$^*$, which could be used to manipulate the scattering length and hence unlock several new experimental possiblities. Previous experimental and theoretical studies for He$^*$ have produced contradictory results. We aimed to resolve this discrepancy with a theoretical search for Feshbach resonances, using a new close-coupled model of He$^*$ collisions in the presence of an external magnetic field. Several resonances were detected and the existing literature discrepancy was resolved. Although none of the resonances identified are readily experimentally useable, an interesting non-Feshbach scattering length variation with magnetic field was observed in heteronuclear collisions, at field strengths that are experimentally accessible.
Understanding and controlling collisions is crucial to the burgeoning field of ultracold molecules. All experiments so far have observed fast loss of molecules from the trap. However, the dominant mechanism for collisional loss is not well understood when there are no allowed 2-body loss processes. Here we experimentally investigate collisional losses of nonreactive ultracold RbCs molecules, and compare our findings with the sticky collision hypothesis that pairs of molecules form long-lived collision complexes. We demonstrate that loss of molecules occupying their rotational and hyperfine ground state is best described by second-order rate equations, consistent with the expectation for complex-mediated collisions, but that the rate is lower than the limit of universal loss. The loss is insensitive to magnetic field but increases for excited rotational states. We demonstrate that dipolar effects lead to significantly faster loss for an incoherent mixture of rotational states.
Significant leaps in the understanding of quantum systems have been driven by the exploration of geometry, topology, dimensionality, and interactions with ultracold atomic ensembles. A system where atoms evolve while confined on an ellipsoidal surface represents a heretofore unexplored geometry and topology. Realizing such an ultracold bubble system (potentially Bose-Einstein condensed) has areas of interest including quantized-vortex flow respecting topological constraints imposed by closed surfaces, new collective modes, and self-interference via free bubble expansion. Large ultracold bubbles, created by inflating smaller condensates, directly tie into Hubble-analog expansion physics. Here, we report observations from the NASA Cold Atom Lab facility aboard the International Space Station of bubbles of ultracold atoms created using a radiofrequency-dressing protocol. We observe a variety of bubble configurations of differing sizes and initial temperature, and explore bubble thermodynamics, demonstrating significant cooling associated with inflation. Additionally, we achieve partial coverings of bubble traps greater than 1 mm in size with ultracold films of inferred few-$mu$m thickness, and we observe the dynamics of shell structures projected into free-evolving harmonic confinement. The observations are part of the first generation of scientific measurements made with ultracold atoms in space, exploiting the benefits of perpetual free-fall to explore gravity-free evolution of quantum systems that are prohibitively difficult to create on Earth. This work points the way to experiments focused on the nature of the Bose-Einstein condensed bubble, the character of its excitations, and the role of topology in its evolution; it also ushers in an era of orbital microgravity quantum-gas physics.
Radiofrequency (RF)-dressed potentials are a promising technique for manipulating atomic mixtures, but so far little work has been undertaken to understand the collisions of atoms held within these traps. In this work, we dress a mixture of 85Rb and 87Rb with RF radiation, characterize the inelastic loss that occurs, and demonstrate species-selective manipulations. Our measurements show the loss is caused by two-body 87Rb+85Rb collisions, and we show the inelastic rate coefficient varies with detuning from the RF resonance. We explain our observations using quantum scattering calculations, which give reasonable agreement with the measurements. The calculations consider magnetic fields both perpendicular to the plane of RF polarization and tilted with respect to it. Our findings have important consequences for future experiments that dress mixtures with RF fields.
We demonstrate microwave dressing on ultracold, fermionic ${}^{23}$Na${}^{40}$K ground-state molecules and observe resonant dipolar collisions with cross sections exceeding three times the $s$-wave unitarity limit. The origin of these collisions is the resonant alignment of the approaching molecules dipoles along the intermolecular axis, which leads to strong attraction. We explain our observations with a conceptually simple two-state picture based on the Condon approximation. Furthermore, we perform coupled-channels calculations that agree well with the experimentally observed collision rates. While collisions are observed here as laser-induced loss, microwave dressing on chemically stable molecules trapped in box potentials may enable the creation of strongly interacting dipolar gases of molecules.
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