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Register a new userMagnetic frustration in the context of pseudo-dipolar ionic disorder
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We consider an alternative to the usual spin glass paradigm for disordered magnetism, consisting of the previously unstudied combination of frustrated magnetic interactions and pseudo-dipolar disorder in spin positions. We argue that this model represents a general limiting case for real systems as well as a realistic model for certain binary fluorides and oxides. Furthermore, it is of great relevance to the highly topical subjects of the Coulomb phase and `charge ice. We derive an analytical solution for the ground state phase diagram of a model system constructed in this paradigm and identify magnetic phases that remain either disordered or partially ordered even at zero temperature. These phases are of a hitherto unobserved type, but may be broadly classified as either `spin liquids or `semi-spin liquids in contrast to the usual spin glass or semi-spin glass. Numerical simulations are used to show that the spin liquid phase exhibits no spin glass transition at finite temperature, despite the combination of frustration and disorder. By mapping onto a model of uncoupled loops of Ising spins, we show that the magnetic structure factor of this phase acts, in the limit $Trightarrow0$, as a sensitive probe of the positional disorder correlations. We suggest that this result can be generalized to more complex systems, including experimental realizations of canonical spin glass models.
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Iron, cobalt and nickel nanoparticles, grown in the gas phase, are known to arrange in chains and bracelet-like rings due to the long-range dipolar interaction between the ferromagnetic (or super-paramagnetic) particles. We investigate the dynamics and thermodynamics of such magnetic dipolar nanoparticles for low densities using molecular dynamics simulations and analyze the influence of temperature and external magnetic fields on two- and three-dimensional systems. The obtained phase diagrams can be understood by using simple energetic arguments.
One of the most remarkable examples of emergent quasi-particles, is that of the fractionalization of magnetic dipoles in the low energy configurations of materials known as spin ice, into free and unconfined magnetic monopoles interacting via Coulombs 1/r law [Castelnovo et. al., Nature, 451, 42-45 (2008)]. Recent experiments have shown that a Coulomb gas of magnetic charges really does exist at low temperature in these materials and this discovery provides a new perspective on otherwise largely inaccessible phenomenology. In this paper, after a review of the different spin ice models, we present detailed results describing the diffusive dynamics of monopole particles starting both from the dipolar spin ice model and directly from a Coulomb gas within the grand canonical ensemble. The diffusive quasi-particle dynamics of real spin ice materials within quantum tunneling regime is modeled with Metropolis dynamics, with the particles constrained to move along an underlying network of oriented paths, which are classical analogues of the Dirac strings connecting pairs of Dirac monopoles.
We computationally study the frustrated magnetic configurations of a thin soft magnetic layer with the boundary condition fixed by underlying hard magnets. Driven by geometrical constraints and external magnetic field, transitions between frustrated energy minima result in magnetic hysteretic behavior. The presence of soft-magnet introduces strong undulations in the energy landscape in a length scale set by the magnetic property of the soft magnet. We propose a possible use of the phenomena to locally control the movement of magnetic nanoparticles.
It has been recently proven that new types of bulk, local order can ensue due to frustrated boundary condition, that is, periodic boundary conditions with an odd number of lattice sites and anti-ferromagnetic interactions. For the quantum XY chain in zero external fields, the usual antiferromagnetic order has been found to be replaced either by a mesoscopic ferromagnet or by an incommensurate AFM order. In this work we examine the resilience of these new types of orders against a defect that breaks the translational symmetry of the model. We find that, while a ferromagnetic defect restores the traditional, staggered order, an AFM one stabilizes the incommensurate order. The robustness of the frustrated order to certain kinds of defects paves the way for its experimental observability.
We present the observation of glass-like dynamic correlations of mobile mercury ions in the ionic conductor Cu2HgI4, detected in both NMR and nonlinear conductivity experiments. The results show that dynamic cooperativity appears in systems seemingly unrelated to glassy and soft arrested materials. A simple kinetic two-component model is proposed, which seems to provide a good description of the cooperative ionic dynamics.
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