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Register a new userTheory of a.c. spin current noise and spin conductance through a quantum dot in the Kondo regime I: The equilibrium case
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We analyze the equilibrium frequency-dependent spin current noise and spin conductance through a quantum dot in the local moment regime. Spin current correlations behave markedly differently from charge correlations. Equilibrium spin correlations are characterized by two universal scaling functions in the absence of an external field: one of them is related to charge correlations, while the other one describes cross-spin correlations. We characterize these functions using a combination of perturbative and non-perturbative methods. We find that at low temperatures spin cross-correlations are suppressed at frequencies below the Kondo scale, $T_K$, and a dynamical spin accumulation resonance is found at the Kondo energy, $omega sim T_K$. At higher temperatures, $T>T_K$, surprising low-frequency anomalies related to overall spin conservation appear in the spin noise and spin conductance, and the Korringa rate is shown to play a distinguished role. The transient spin current response also displays universal and singular properties.
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Spin and charge transport through a quantum dot coupled to external nonmagnetic leads is analyzed theoretically in terms of the non-equilibrium Green function formalism based on the equation of motion method. The dot is assumed to be subject to spin and charge bias, and the considerations are focused on the Kondo effect in spin and charge transport. It is shown that the differential spin conductance as a function of spin bias reveals a typical zero-bias Kondo anomaly which becomes split when either magnetic field or charge bias are applied. Significantly different behavior is found for mixed charge/spin conductance. The influence of electron-phonon coupling in the dot on tunneling current as well as on both spin and charge conductance is also analyzed.
We consider the non-equilibrium zero frequency noise generated by a temperature gradient applied on a device composed of two normal leads separated by a quantum dot. We recall the derivation of the scattering theory for non-equilibrium noise for a general situation where both a bias voltage and a temperature gradient can coexist and put it in a historical perspective. We provide a microscopic derivation of zero frequency noise through a quantum dot based on a tight binding Hamiltonian, which constitutes a generalization of the pioneering work of Caroli et al. for the current obtained in the context of the Keldysh formalism. For a single level quantum dot, the obtained transmission coefficient entering the scattering formula for the non-equilibrium noise corresponds to a Breit-Wigner resonance. We compute the delta-$T$ noise as a function of the dot level position, and of the dot level width, in the Breit-Wigner case, for two relevant situations which were considered recently in two separate experiments. In the regime where the two reservoir temperatures are comparable, our gradient expansion shows that the delta-$T$ noise is dominated by its quadratic contribution, and is minimal close to resonance. In the opposite regime where one reservoir is much colder, the gradient expansion fails and we find the noise to be typically linear in temperature before saturating. In both situations, we conclude with a short discussion of the case where both a voltage bias and a temperature gradient are present, in order to address the potential competition with thermoelectric effects.
We report selective injection of both spin-up and spin-down single electrons into a quantum dot (QD) from spin-polarized non-equilibrium quantum Hall edge channels (ECs) generated by selective transmission of spin-resolved ECs using a surface gate placed at a distance from the QD. We change the spin polarization of non-equilibrium ECs by changing the bias voltages applied to different source Ohmic contacts. The efficiency of spin-up electron injection reaches 0.5, which is approximately 0.2 higher than that induced by spin-dependent tunnel coupling between QD and ECs. On the other hand, the efficiency of spin-down electron injection reaches 0.4. In addition, we rectify the underestimation of the efficiency of spin filtering for equilibrium ECs by numerically subtracting the contribution of the excited states in the QD. The obtained spin-filtering efficiency is higher than that evaluated from the raw experimental data and increases with magnetic field as expected with the increase in the spatial separation between ECs.
The current emission noise of a carbon nanotube quantum dot in the Kondo regime is measured at frequencies $ u$ of the order or higher than the frequency associated with the Kondo effect $k_B T_K/h$, with $T_K$ the Kondo temperature. The carbon nanotube is coupled via an on-chip resonant circuit to a quantum noise detector, a superconductor-insulator-superconductor junction. We find for $h u approx k_B T_K$ a Kondo effect related singularity at a voltage bias $eV approx h u $, and a strong reduction of this singularity for $h u approx 3 k_B T_K$, in good agreement with theory. Our experiment constitutes a new original tool for the investigation of the non-equilibrium dynamics of many-body phenomena in nanoscale devices.
We analyze the equilibrium and non-equilibrium frequency-dependent spin current noise and spin conductance through a quantum dot in the local moment regime. Spin current correlations are shown to behave markedly differently from charge correlations: Equilibrium spin cross-correlations are suppressed at frequencies below the Kondo scale, and are characterized by a universal function that we determine numerically for zero temperature. For asymmetrical quantum dots dynamical spin accumulation resonance is found for frequencies of the order of the Kondo energy. At higher temperatures surprising low-frequency anomalies related to overall spin conservation appear.
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