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Register a new userDoppler-free two-photon resonances for atom detection and sum frequency stabilization
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We investigate the excitation of the 5D_{5/2} level in Rb atoms using counter-propagating laser beams, which are nearly resonant to the one-photon 5S_{1/2} - 5P_{3/2} and 5P_{3/2} - 5D_{5/2} transitions, ensuring that a sum of the optical frequencies corresponds to the 5S_{1/2} - 5D_{5/2} transition. The excitation produced by two-photon and step-wise processes is detected via spontaneously emitted fluorescence at 420 nm arising from the 6P_{3/2} - 5S_{1/2} transition. The dependences of blue fluorescence intensity on atomic density and laser detuning from the intermediate 5P_{3/2} level have been investigated. The sensitivity of the frequency detuned bi-chromatic scheme for atom detection has been estimated. A novel method for sum frequency stabilization of two free-running lasers has been suggested and implemented using two-photon Doppler-free fluorescence and polarization resonances.
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The $3p^{4}$ $^{3}$P$_{J}$ - $3p^{3}4p$ $^{3}$P$_{J}$ transition in the sulphur atom is investigated in a precision two-photon excitation scheme under Doppler-free and collision-free circumstances yielding an absolute accuracy of 0.0009 cm$^{-1}$, using a narrowband pulsed laser. This verifies and improves the level separations between amply studied odd parity levels with even parity levels in S I. An improved value for the $^{3}$P$_{2}$ - $^{3}$P$_{1}$ ground state fine structure splitting is determined at $396.0564$ (7) cm$^{-1}$. A $^{34}$S - $^{32}$S atomic isotope shift was measured from combining time-of-flight mass spectrometry with laser spectroscopy.
Collisions with background gas particles can shift the resonance frequencies of atoms in atomic clocks. The internal quantum states of atoms can also become entangled with their motional states due to the recoil imparted by a collision, which leads to a further shift of the clock frequency through the relativistic Doppler shift. It can be complicated to evaluate the Doppler and collisional frequency shifts for clock atoms in such entangled states, but estimates of these shifts are essential in order to improve the accuracy of optical atomic clocks. We present a formalism that describes collisions and relativistic Doppler shifts in a unified manner, and can therefore be used to accurately estimate collisional frequency shifts in trapped-atom clocks.
Spontaneous parametric down conversion (PDC), in the perturbative limit, can be considered as a probabilistic splitting of one input photon into two output photons. Conversely, sum-frequency generation (SFG) implements the reverse process of combining two input photons into one. Here we show that a single-photon projective measurement in the temporal-mode basis of the output photon of a two-photon SFG process effects a generalized measurement on the input two-photon state. We describe the positive-operator-valued measure (POVM) associated with such a measurement, and show that its elements are proportional to the two-photon states produced by the time-reversed PDC process. Such a detection acts as a joint measurement on two photons, and is thus an important component of many quantum information processing protocols relying on photonic entanglement. Using the retrodictive approach, we analyze the properties of the two-photon POVM that are relevant for quantum protocols exploiting two-photon states and measurements.
We propose and demonstrate a scheme to enable Doppler compensation within optical cavities for atom interferometry at significantly increased mode diameters. This has the potential to overcome the primary limitations in cavity enhancement for atom interferometry, circumventing the cavity linewidth limit and enabling mode filtering, power enhancement, and a large beam diameter simultaneously. This approach combines a magnified linear cavity with an intracavity Pockels cell. The Pockels cell introduces a voltage tunable birefringence allowing the cavity mode frequencies to track the Raman lasers as they scan to compensate for gravitationally induced Doppler shifts, removing the dominant limitation of current cavity enhanced systems. A cavity is built to this geometry and shown to simultaneously realize the capability required for Doppler compensation, with a 5.04~mm $1/e^{2}$ diameter beam waist and an enhancement factor of $>$5x at a finesse of 35. Furthermore, this has a tunable Gouy phase, allowing the suppression of higher order spatial modes and the avoidance of regions of instability. This approach can therefore enable enhanced contrast and longer atom interferometry times while also enabling the key features of cavity enhanced atom interferometry, power enhancement and the reduction of aberrations. This is relevant to future reductions in the optical power requirement of quantum technology, or in providing enhanced performance for atom interferometers targeting fundamental science.
Gravitational waves imprint apparent Doppler shifts on the frequency of photons propagating between an emitter and detector of light. This forms the basis of a method to detect gravitational waves using Doppler velocimetry between pairs of satellites. Such detectors, operating in the milli-hertz gravitational frequency band, could lead to the direct detection of gravitational waves. The crucial component in such a detector is the frequency standard on board the emitting and receiving satellites. We point out that recent developments in atomic frequency standards have led to devices that are approaching the sensitivity required to detect gravitational waves from astrophysically interesting sources. The sensitivity of satellites equipped with optical frequency standards for Doppler velocimetry is examined, and a design for a robust, space-capable optical frequency standard is presented.
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