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Register a new userJamming phase diagram of athermal emulsions with short-range attraction
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Using confocal microscopy we investigate the effect of attraction on the packing of polydisperse emulsions under gravity. We find that the distributions of neighbors, coordination number, and local packing fraction as a function of attraction are captured by recently proposed geometrical modeling and statistical mechanics approaches to granular matter. This extends the range of applicability of these tools to polydisperse, attractive jammed packings. Furthermore, the dependence of packing density and average coordination number on the strength of attraction provides the first experimental test of a phase diagram of athermal jammed particles. The success of these theoretical frameworks in describing a new class of systems gives support to the much-debated statistical physics of jammed matter.
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We perform numerical simulations of athermal repulsive frictionless disks and spheres in two and three spatial dimensions undergoing cyclic quasi-static simple shear to investigate particle-scale reversible motion. We identify three classes of steady-state dynamics as a function of packing fraction phi and maximum strain amplitude per cycle gamma_{rm max}. Point-reversible states, where particles do not collide and exactly retrace their intra-cycle trajectories, occur at low phi and gamma_{rm max}. Particles in loop-reversible states undergo numerous collisions and execute complex trajectories, but return to their initial positions at the end of each cycle. Loop-reversible dynamics represents a novel form of self-organization that enables reliable preparation of configurations with specified structural and mechanical properties over a broad range of phi from contact percolation to jamming onset at phi_J. For sufficiently large phi and gamma_{rm max}, systems display irreversible dynamics with nonzero self-diffusion.
We study the elasto-plastic behavior of dense attractive emulsions under mechanical perturbation. The attraction is introduced through non-specific depletion interactions between the droplets and is controlled by changing the concentration of surfactant micelles in the continuous phase. We find that such attractive forces are not sufficient to induce any measurable modification on the scalings between the local packing fraction and the deformation of the droplets. However, when the emulsions are flown through 2D microfluidic constrictions, we uncover a measurable effect of attraction on their elasto-plastic response. Indeed, we measure higher levels of deformation inside the constriction for attractive droplets. In addition, we show that these measurements correlate with droplet rearrangements that are spatially delayed in the constriction for higher attraction forces.
We derive exact results for displacement fields that develop as a response to external pinning forces in two dimensional athermal networks. For a triangular lattice arrangement of particles interacting through soft potentials, we develop a Greens function formalism which we use to derive exact results for displacement fields produced by localized external forces. We show that in the continuum limit the displacement fields decay as $1/r$ at large distances $r$ away from a force dipole. Finally, we extend our formulation to study correlations in the displacement fields produced by the external pinning forces. We show that uncorrelated pinned forces at each vertex give rise to long-range correlations in displacements in athermal systems, with a non-trivial system size dependence. We verify our predictions with numerical simulations of athermal networks in two dimensions.
We study numerically and analytically a model of self-propelled polar disks on a substrate in two dimensions. The particles interact via isotropic repulsive forces and are subject to rotational noise, but there is no aligning interaction. As a result, the system does not exhibit an ordered state. The isotropic fluid phase separates well below close packing and exhibits the large number fluctuations and clustering found ubiquitously in active systems. Our work shows that this behavior is a generic property of systems that are driven out of equilibrium locally, as for instance by self propulsion.
Self-organization, and transitions from reversible to irreversible behaviour, of interacting particle assemblies driven by externally imposed stresses or deformation is of interest in comprehending diverse phenomena in soft matter. They have been investigated in a wide range of systems, such as colloidal suspensions, glasses, and granular matter. In different density and driving regimes, such behaviour is related to yielding of amorphous solids, jamming, and memory formation, emph{etc.} How these phenomena are related to each other has not, however, been much studied. In order to obtain a unified view of the different regimes of behaviour, and transitions between them, we investigate computationally the response of soft sphere assemblies to athermal cyclic shear deformation over a wide range of densities and amplitudes of shear deformation. Cyclic shear deformation induces transitions from reversible to irreversible behaviour in both unjammed and jammed soft sphere packings. Well above isotropic jamming density ($bf{phi_J}$), this transition corresponds to yielding. In the vicinity of the jamming point, up to a higher density limit we designate ${bf phi_J^{cyc}}$, an unjammed phase emerges between a localised, emph{absorbing} phase, and a diffusive, {emph irreversible} phase. The emergence of the unjammed phase signals the shifting of the jamming point to higher densities as a result of annealing, and opens a window where shear jamming becomes possible for frictionless packings. Below $bf{phi_J}$, two distinct localised states, termed point and loop reversibile, are observed. We characterise in detail the different regimes and transitions between them, and obtain a unified density-shear amplitude phase diagram.
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