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Register a new userPlanar CuO_2 hole density estimation in multilayered high-T_c cuprates
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We report that planar CuO_2 hole densities in high-T_c cuprates are consistently determined by the Cu-NMR Knight shift. In single- and bi-layered cuprates, it is demonstrated that the spin part of the Knight shift K_s(300 K) at room temperature monotonically increases with the hole density $p$ from underdoped to overdoped regions, suggesting that the relationship of K_s(300 K) vs. p is a reliable measure to determine p. The validity of this K_s(300 K)-p relationship is confirmed by the investigation of the p-dependencies of hyperfine magnetic fields and of spin susceptibility for single- and bi-layered cuprates with tetragonal symmetry. Moreover, the analyses are compared with the NMR data on three-layered Ba_2Ca_2Cu_3O_6(F,O)_2, HgBa_2Ca_2Cu_3O_{8+delta}, and five-layered HgBa_2Ca_4Cu_5O_{12+delta}, which suggests the general applicability of the K_s(300 K)-p relationship to multilayered compounds with more than three CuO_2 planes. We remark that the measurement of K_s(300 K) enables us to separately estimate p for each CuO_2 plane in multilayered compounds, where doped hole carriers are inequivalent between outer CuO_2 planes and inner CuO_2 planes.
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We present a study of the in-plane and out-of-plane magnetoresistance (MR) in heavily-underdoped, antiferromagnetic YBa_{2}Cu_{3}O_{6+x}, which reveals a variety of striking features. The in-plane MR demonstrates a d-wave-like anisotropy upon rotating the magnetic field H within the ab plane. With decreasing temperature below 20-25 K, the system acquires memory: exposing a crystal to the magnetic field results in a persistent in-plane resistivity anisotropy. The overall features can be explained by assuming that the CuO_2 planes contain a developed array of stripes accommodating the doped holes, and that the MR is associated with the field-induced topological ordering of the stripes.
High-temperature superconducting cuprates are distinguished by an enigmatic pseudogap which opens near optimal doping where the superconducting transition temperature is highest. Key questions concern its origin and whether it is essential in any way to superconductivity. Recent field-induced normal-state transport experiments on hole-doped cuprates have measured abrupt changes in the doping dependent Hall number and resistivity, consistent with a drop in carrier density from $1+p$ to $p$ holes per copper atom, on entering the pseudogap phase. In this work the change in resistivity is analyzed in terms of an antiferromagnetic-order-induced Fermi surface reconstruction model that has already successfully described the Hall number. In order for this model to describe the resistivity we find that the zero-temperature mean free path must also drop abruptly in proportion to the size of the Fermi surface. This suggests that intrapocket scattering underlies the observed upturn in resistivity in the pseudogap state.
Cuprate superconductors have long been known to exhibit an energy gap that persists high above the superconducting transition temperature ($T_c$). Debate has continued now for decades as to whether it is a precursor superconducting gap or a pseudogap arising from some competing correlation. Failure to resolve this has arguably delayed explaining the origins of superconductivity in these highly complex materials. Here we effectively settle the question by calculating a variety of thermodynamic and spectroscopic properties, exploring the effect of a temperature-dependent pair-breaking term in the self-energy in the presence of pairing interactions that persist well above $T_c$. We start by fitting the detailed temperature-dependence of the electronic specific heat and immediately can explain its hitherto puzzling field dependence. Taking this same combination of pairing temperature and pair-breaking scattering we are then able to simultaneously describe in detail the unusual temperature and field dependence of the superfluid density, tunneling, Raman and optical spectra, which otherwise defy explanation in terms a superconducting gap that closes conventionally at $T_c$. These findings demonstrate that the gap above $T_c$ in the overdoped regime likely originates from incoherent superconducting correlations, and is distinct from the competing-order pseudogap that appears at lower doping.
Here we reply to Farids comment.
We present a Boltzmann equation analysis of the transport properties of a model of electrons with a lifetime which is short everywhere except near the Brillouin zone diagonals. The anomalous lifetime is directly implied by photoemission and c-axis transport data. We find quantitative agreement between calculations and ac and dc longitudinal and Hall resistivity, but the predicted longitudinal magnetoresistance disagrees with experiment. A possible microscopic origin of the anomalous lifetime is discussed
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