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Specific heat across the superconducting dome in the cuprates

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 Added by Elisabeth Nicol
 Publication date 2010
  fields Physics
and research's language is English




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The specific heat of the superconducting cuprates is calculated over the entire phase diagram. A d-wave BCS approach based on the large Fermi surface of Fermi liquid and band structure theory provides a good description of the overdoped region. At underdoping it is essential to include the emergence of a second energy scale, the pseudogap and its associated Gutzwiller factor, which accounts for a reduction in the coherent piece of the electronic Greens function due to increased correlations as the Mott insulating state is approached. In agreement with experiment, we find that the slope of the linear in T dependence of the low temperature specific heat rapidly increases above optimum doping while it is nearly constant below optimum. Our theoretical calculations also agree with recent data on Bi$_2$Sr$_{2-rm x}$La$_{rm x}$CuO$_{6+delta}$ for which the normal state is accessed through the application of a large magnetic field. A quantum critical point is located at a doping slightly below optimum.



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329 - L. Dudy , A. Krapf , H. Dwelk 2010
We report characterization results by energy dispersive x-ray analysis and AC-susceptibility for a statistically relevant number of single layer Bi-cuprate single crystals. We show that the two structurally quite different modifications of the single-layered Bi-cuprate, namely (La,Pb=0.4)-Bi2201 and La-Bi2201, exhibit anomalies in the superconducting transition temperature at certain hole doping, e.g. at 1/8 holes per Cu. These doping values agree well with the magic doping fractions found in the temperature dependent resistance of LSCO by Komiya et al. This new set of findings suggests that all these anomalies are generic for the hole-doped high-temperature superconductors.
Understanding the thermodynamic properties of high-$T_c$ cuprate superconductors is a key step to establish a satisfactory theory of these materials. The electronic specific heat is highly unconventional, distinctly non-BCS, with remarkable doping-dependent features extending well beyond $T_c$. The pairon concept, bound holes in their local antiferromagnetic environment, has successfully described the tunneling and photoemission spectra. In this article, we show that the model explains the distinctive features of the entropy and specific heat throughout the temperature-doping phase diagram. Their interpretation connects unambiguously the pseudogap, existing up to $T^*$, to the superconducting state below $T_c$. In the underdoped case, the specific heat is dominated by pairon excitations, following Bose statistics, while with increasing doping, both bosonic excitations and fermionic quasiparticles coexist.
Hole doped cuprates show a superconducting critical temperature $T_c$ which follows an universal dome-shaped behavior as function of doping. It is believed that the origin of superconductivity in cuprates is entangled with the physics of the pseudogap phase. An open discussion is whether the source of superconductivity is the same that causes the pseudogap properties. The $t$-$J$ model treated in large-N expansion shows $d$-wave superconductivity triggered by non-retarded interactions, and an instability of the paramagnetic state to a flux phase or $d$-wave charge density wave ($d$-CDW) state. In this paper we show that self-energy effects near $d$-CDW instability may lead to a dome-shaped behavior of $T_c$. In addition, it is also shown that these self-energy contributions may describe several properties observed in the pseudogap phase. In this picture, although fluctuations responsible for the pseudogap properties leads to a dome-shaped behavior, they are not involved in pairing which is mainly non-retarded.
We investigate the specific heat of ultra-pure single crystals of Sr2RuO4, a leading candidate of a spin-triplet superconductor. We for the first time obtained specific-heat evidence of the first-order superconducting transition below 0.8 K, namely divergent-like peaks and clear hysteresis in the specific heat at the upper critical field. The first-order transition occurs for all in-plane field directions. The specific-heat features for the first-order transition are found to be highly sensitive to sample quality; in particular, the hysteresis becomes totally absent in a sample with slightly lower quality. These thermodynamic observations provide crucial bases to understand the unconventional pair-breaking effect responsible for the first-order transition.
The Berezinskii-Kosterlitz-Thouless (BKT) transition is expected to have a clear signature on the specific heat. The singularity at the transition temperature $T_{BKT}$ is predicted to be immeasurable, and a broad non-universal peak is expected at $T>T_{BKT}$. Up to date this has not been observed in two-dimensional superconductors. We use a unique highly sensitive technique to measure the specific heat of ultrathin Pb films. We find that thick films exhibit a specific heat jump at $T_C$ that is consistent with BCS theory. As the film thickness is reduced below the superconducting coherence length and the systems enters the 2D limit the specific heat reveals BKT-like behavior. We discuss these observations in the framework of the continuous BCS-BKT crossover as a function of film thickness.
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