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Supplemental Material for Paper Metallization of Nanofilms in Strong Adiabatic Electric Fields

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 Added by Maxim Durach
 Publication date 2010
  fields Physics
and research's language is English




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We introduce an effect of metallization of dielectric nanofilms by strong, adiabatically varying electric fields. The metallization causes optical properties of a dielectric film to become similar to those of a plasmonic metal (strong absorption and negative permittivity at low optical frequencies). The is a quantum effect, which is exponentially size-dependent, occurring at fields on the order of 0.1 V/A and pulse durations ranging from ~ 1 fs to ~ 10 ns for film thickness 3 to 10 nm.



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We introduce an effect of metallization of dielectric nanofilms by strong, adiabatically varying electric fields. The metallization causes optical properties of a dielectric film to become similar to those of a plasmonic metal (strong absorption and negative permittivity at low optical frequencies). The is a quantum effect, which is exponentially size-dependent, occurring at fields on the order of 0.1 V/A and pulse durations ranging from ~ 1 fs to ~ 10 ns for film thickness 3 to 10 nm.
We predict a dynamic metallization effect where an ultrafast (single-cycle) optical pulse with a field less or on the order of 1 V/Angstrom causes plasmonic metal-like behavior of a dielectric film with a few-nm thickness. This manifests itself in plasmonic oscillations of polarization and a significant population of the conduction band evolving on a femtosecond time scale. These phenomena are due a combination of both adiabatic (reversible) and diabatic (for practical purposes irreversible) pathways.
Helical modes, conducting opposite spins in opposite directions, are shown to exist in metallic armchair nanotubes in an all-electric setup. This is a consequence of the interplay between spin-orbit interaction and strong electric fields. The helical regime can also be obtained in chiral metallic nanotubes by applying an additional magnetic field. In particular, it is possible to obtain helical modes at one of the two Dirac points only, while the other one remains gapped. Starting from a tight-binding model we derive the effective low-energy Hamiltonian and the resulting spectrum.
We study the effect of a strong electric field on the fluctuation conductivity within the time-dependent Ginzburg-Landau theory for the case of arbitrary dimension. Our results are based on the analytical derivation of the velocity distribution law for the fluctuation Cooper pairs, from the Boltzmann equation. Special attention is drawn to the case of small nonlinearity of conductivity, which can be investigated experimentally. We obtain a general relation between the nonlinear conductivity and the temperature derivative of the linear Aslamazov-Larkin conductivity, applicable to any superconductor. For the important case of layered superconductors we derive an analogous relation between the small nonlinear correction for the conductivity and the fluctuational magnetoconductivity. On the basis of these relations we provide new experimental methods for determining both the lifetime constant of metastable Cooper pairs above T_c and the coherence length. A systematic investigation of the 3rd harmonic of the electric field generated by a harmonic current can serve as an alternative method for the examination of the metastable Cooper-pair relaxation time.
163 - Rong-Bin Chen , Chin-Wei Chiu , 2016
Monolayer tinene presents rich absorption spectra in electric fields. There are three kinds of special structures, namely shoulders, logarithmically symmetric peaks and asymmetric peaks in the square-root form, corresponding to the optical excitations of the extreme points, saddle points and constant-energy loops. With the increasing field strength, two splitting shoulder structures, which are dominated by the parabolic bands of ${5p_z}$ orbitals, come to exist because of the spin-split energy bands. The frequency of threshold shoulder declines to zero and then linearly grows. The third shoulder at ${0.75 sim 0.85}$ eV mainly comes from (${5p_x,5p_y}$) orbitals. The former and the latter orbitals, respectively, create the saddle-point symmetric peaks near the M point, while they hybridize with one another to generate the loop-related asymmetric peaks. Tinene quite differs from graphene, silicene, and germanene. The special relationship among the multi-orbital chemical bondings, spin-orbital couplings and Coulomb potentials accounts for the feature-rich optical properties.
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