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Register a new userSwitching Casimir forces with Phase Change Materials
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We demonstrate here a controllable variation in the Casimir force. Changes in the force of up to 20% at separations of ~100 nm between Au and AgInSbTe (AIST) surfaces were achieved upon crystallization of an amorphous sample of AIST. This material is well known for its structural transformation, which produces a significant change in the optical properties and is exploited in optical data storage systems. The finding paves the way to the control of forces in nanosystems, such as micro- or nanoswitches by stimulating the phase change transition via localized heat sources.
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A stable suspension of nanoscale particles due to the Casimir force is of great interest for many applications such as sensing, non-contract nano-machines. However, the suspension properties are difficult to change once the devices are fabricated. Vanadium dioxide (VO$_2$) is a phase change material, which undergoes a transition from a low-temperature insulating phase to a high-temperature metallic phase around a temperature of 340 K. In this work, we study Casimir forces between a nanoplate (gold or Teflon) and a layered structure containing a VO$_2$ film. It is found that stable Casimir suspensions of nanoplates can be realized in a liquid environment, and the equilibrium distances are determined, not only by the layer thicknesses but also by the matter phases of VO$_2$. Under proper designs, a switch from quantum trapping of the gold nanoplate (on state) to its release (off state) as a result of the metal-to-insulator transition of VO$_2$, is revealed. On the other hand, the quantum trapping and release of a Teflon nanoplate is found under the insulator-to-metal transition of VO$_2 $. Our findings offer the possibility of designing switchable devices for applications in micro-and nano-electromechanical systems.
We investigate repulsive Casimir force between slabs containing left-handed materials with controllable electromagnetic properties. The sign of Casimir force is determined by the electric and magnetic properties of the materials, and it is shown that the formation of the repulsive force is related to the wave impedances of two slabs. The sign change of the Casimir force as a function of the distance is studied. Special emphasis is put on the restoring Casimir force which may be found to exist between perfectly conducting material and metamaterial slabs. This restoring force is a natural power for the system oscillation in vacuum and also can be used for system stabilization.
Microparticles including paraffin are currently used for textiles coating in order to deaden thermal shocks. We will show that polymer nanoparticles embedded in those microsized capsules allow for decreasing the thermal conductivity of the coating and enhance the protection in the stationary regime. A reasonable volume fraction of polymer nanoparticles reduces the conductivity more than predicted by Maxwell mixing rules. Besides, measurements prove that the polymer nanoparticles do not affect the latent heat and even improve the phase change behaviour as well as the mechanical properties.
Chalcogenide alloys are materials of interest for optical recording and non-volatile memories. We perform ab-initio molecular dynamics simulations aiming at shading light onto the structure of amorphous Ge2Sb2Te5 (GST), the prototypical material in this class. First principles simulations show that amorphous GST obtained by quenching from the liquid phase displays two types of short range order. One third of Ge atoms are in a tetrahedral environment while the remaining Ge, Sb and Te atoms display a defective octahedral environment, reminiscent of cubic crystalline GST.
Ge2Sb2Te5 and related phase change materials are highly unusual in that they can be readily transformed between amorphous and crystalline states using very fast melt, quench, anneal cycles, although the resulting states are extremely long lived at ambient temperature. These states have remarkably different physical properties including very different optical constants in the visible in strong contrast to common glass formers such as silicates or phosphates. This behavior has been described in terms of resonant bonding, but puzzles remain, particularly regarding different physical properties of crystalline and amorphous phases. Here we show that there is a strong competition between ionic and covalent bonding in cubic phase providing a link between the chemical basis of phase change memory property and origins of giant responses of piezoelectric materials (PbTiO3, BiFeO3). This has important consequences for dynamical behavior in particular leading to a simultaneous hardening of acoustic modes and softening of high frequency optic modes in crystalline phase relative to amorphous. This different bonding in amorphous and crystalline phases provides a direct explanation for different physical properties and understanding of the combination of long time stability and rapid switching and may be useful in finding new phase change compositions with superior properties.
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