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Evidence of a photoinduced non-thermal superconducting-to-normal-state phase transition in overdoped Bi$_{2}$Sr$_{2}$Ca$_{0.92}$Y$_{0.08}$Cu$_{2}$O$_{8+delta}$

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 Publication date 2010
  fields Physics
and research's language is English




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Here we report extensive ultrafast time-resolved reflectivity experiments on overdoped Bi$_{2}$Sr$_{2}$Ca$_{1-x}$Y$_x$Cu$_{2}$O$_{8+delta}$ single crystals (T$_C$=78 K) aimed to clarify the nature of the superconducting-to-normal-state photoinduced phase transition. The experimental data show the lack of the quasiparticles decay time divergence at the fluence required to induce this phase transition, in contrast to the thermally-driven phase transition observed at T$_C$ and at variance with recently reported photoinduced charge-density-wave and spin-density-wave to metal phase transitions. Our data demonstrate the non-thermal character of the superconducting-to-normal-state photoinduced phase transition. The data have been analyzed using an ad-hoc developed time-dependent Rothwarf-Taylor model, opening the question on the order of this non-equilibrium phase transition.



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Ultrafast broadband transient reflectivity experiments are performed to study the interplay between the non-equilibrium dynamics of the pseudogap and the superconducting phases in Bi$_{2}$Sr$_{2}$Ca$_{0.92}$Y$_{0.08}$Cu$_{2}$O$_{8+delta}$. Once superconductivity is established the relaxation of the pseudogap proceeds $sim$ 2 times faster than in the normal state, and the corresponding transient reflectivity variation changes sign after $sim$ 0.5 ps. The results can be described by a set of coupled differential equations for the pseudogap and for the superconducting order parameter. The sign and strength of the coupling term suggest a remarkably weak competition between the two phases, allowing their coexistence.
We report an ARPES investigation of the circular dichroism in the first Brillouin zone (BZ) of under- and overdoped Pb-Bi2212 samples. We show that the dichroism has opposite signs for bonding and antibonding components of the bilayer-split CuO-band and is antisymmetric with respect to reflections in both mirror planes parallel to the c-axis. Using this property of the energy and momentum intensity distributions we prove the existence of the bilayer splitting in the normal state of the underdoped compound and compare its value with the splitting in overdoped sample. In agreement with previous studies the magnitude of the interlayer coupling does not depend significantly on doping. We also discuss possible origins of the observed dichroism.
We report a fine tuned doping study of strongly overdoped Bi$_2$Sr$_2$CaCu$_2$O$_{8+delta}$ single crystals using electronic Raman scattering. Combined with theoretical calculations, we show that the doping, at which the normal state pseudogap closes, coincides with a Lifshitz quantum phase transition where the active hole-like Fermi surface becomes electron-like. This conclusion suggests that the microscopic cause of the pseudogap is sensitive to the Fermi surface topology. Furthermore, we find that the superconducting transition temperature is unaffected by this transition, demonstrating that their origins are different on the overdoped side.
The Josephson Plasma Resonance is used to study the c-axis supercurrent in the superconducting state of underdoped Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+delta}$ with varying degrees of controlled point-like disorder, introduced by high-energy electron irradiation. As disorder is increased, the Josephson Plasma frequency decreases proportionally to the critical temperature. The temperature dependence of the plasma frequency does not depend on the irradiation dose, and is in quantitative agreement with a model for quantum fluctuations of the superconducting phase in the CuO$_{2}$ layers.
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We estimated the ratios of $^{63}$Cu hyperfine coupling constants in the double-layer high-$T_mathrm{c}$ superconductor HgBa$_2$CaCu$_2$O$_{6+delta}$ from the anisotropies in Cu nuclear spin-lattice relaxation rates and spin Knight shifts to study the nature of the ultraslow fluctuations causing the $T_2$ anomaly in the Cu nuclear spin-echo decay. The ultraslow fluctuations may come from uniform magnetic fluctuations spread around the wave vector $q$ = 0, otherwise the electric origins.
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