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Register a new userPrecise study of the resonance at Q0=(1,0,0) in URu2Si2
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New inelastic neutron scattering experiments have been performed on URu2Si2 with special focus on the response at Q0=(1,0,0), which is a clear signature of the hidden order (HO) phase of the compound. With polarized inelastic neutron experiments, it is clearly shown that below the HO temperature (T0 = 17.8 K) a collective excitation (the magnetic resonance at E0 approx 1.7 meV) as well as a magnetic continuum co-exist. Careful measurements of the temperature dependence of the resonance lead to the observation that its position shifts abruptly in temperature with an activation law governed by the partial gap opening and that its integrated intensity has a BCS-type temperature dependence. Discussion with respect to recent theoretical development is made.
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We focus on inelastic neutron scattering in $URu_2Si_2$ and argue that observed gap in the fermion spectrum naturally leads to the spin feature observed at energies $omega_{res} = 4-6 meV$ at momenta at $bQ^* = (1pm 0.4, 0,0)$. We discuss how spin features seen in $URu_2Si_2$ can indeed be thought of in terms of {em spin resonance} that develops in HO state and is {em not related} to superconducting transition at 1.5K. In our analysis we assume that the HO gap is due to a particle-hole condensate that connects nested parts of the Fermi surface with nesting vector $bf{Q}^* $. Within this approach we can predicted the behavior of the spin susceptibility at $bQ^*$ and find it to be is strikingly similar to the phenomenology of resonance peaks in high-T$_c$ and heavy fermion superconductors. The energy of the resonance peak scales with $T_{HO}$ $omega_{res} simeq 4 k_BT_{HO}$. We discuss observable consequences spin resonance will have on neutron scattering and local density of states.
Simultaneous neutron-scattering and thermal expansion measurements on the heavy-fermion superconductor URu2Si2 under hydrostatic pressure of 0.67 GPa have been performed in order to detect the successive paramagnetic, hidden order, and large moment antiferromagnetic phases on cooling. The temperature dependence of the sharp low energy excitation at the wavevector Q_0=(100) shows that this excitation is clearly a signature of the hidden order state. In the antiferromagnetic phase, this collective mode disappears. The higher energy excitation at the incommensurate wavevector Q_1=(1.4,0,0) persists in the antiferromagnetic phase but increases in energy. The collapse of the inelastic neutron scattering at Q_0 coincides with the previous observation of the disappearance of superconductivity.
To resolve the nature of the hidden order below 17.5,K in the heavy fermion compound URu$_2$Si$_2$, identifying which symmetries are broken below the hidden order transition is one of the most important steps. Several recent experiments on the electronic structure have shown that the Fermi surface in the hidden order phase is quite close to the result of band-structure calculations within the framework of itinerant electron picture assuming the antiferromagnetism. This provides strong evidence for the band folding along the c-axis with the ordering vector of $(0,0,1)$, corresponding to broken translational symmetry. In addition to this, there is growing evidence for fourfold rotational symmetry breaking in the hidden-order phase from measurements of the in-plane magnetic anisotropy and the effective mass anisotropy in the electronic structure, as well as the orthorhombic lattice distortion. This broken fourfold symmetry gives a stringent constraint that the symmetry of the hidden order parameter should belong to the degenerate $E$-type irreducible representation. We also discuss a possibility that time reversal symmetry is also broken, which further narrows down the order parameter that characterizes the hidden order.
We report 29Si nuclear magnetic resonance measurements of single crystals and aligned powders of URu2Si2 under pressure in the hidden order and paramagnetic phases. We find that the Knight shift decreases with applied pressure, consistent with previous measurements of the static magnetic susceptibility. Previous measurements of the spin lattice relaxation time revealed a partial suppression of the density of states below 30 K. This suppression persists under pressure, and the onset temperature is mildly enhanced.
Novel electronic states resulting from entangled spin and orbital degrees of freedom are hallmarks of strongly correlated f-electron systems. A spectacular example is the so-called hidden-order phase transition in the heavy-electron metal URu2Si2, which is characterized by the huge amount of entropy lost at T_{HO}=17.5K. However, no evidence of magnetic/structural phase transition has been found below T_{HO} so far. The origin of the hidden-order phase transition has been a long-standing mystery in condensed matter physics. Here, based on a first-principles theoretical approach, we examine the complete set of multipole correlations allowed in this material. The results uncover that the hidden-order parameter is a rank-5 multipole (dotriacontapole) order with nematic E^- symmetry, which exhibits staggered pseudospin moments along the [110] direction. This naturally provides comprehensive explanations of all key features in the hidden-order phase including anisotropic magnetic excitations, nearly degenerate antiferromagnetic-ordered state, and spontaneous rotational-symmetry breaking.
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