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Register a new userPenetration depth of electron-doped-infinite-layer Sr$_{0.88}$La$_{0.12}$CuO$_{2+x}$ thin films
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The in-plane penetration depth of Sr$_{0.88}$La$_{0.12}$CuO$_{2+x}$ thin films at various doping obtained from oxygen reduction has been measured, using AC susceptibility measurements. For the higher doping samples, the superfluid density deviates strongly from the s-wave behavior, suggesting, in analogy with other electron-doped cuprates, a contribution from a nodal hole pocket, or a small gap on the Fermi surface such as an anisotropic s-wave order parameter. The low value of the superfluid densities, likely due to a strong doping-induced disorder, places the superconducting transition of our samples in the phase-fluctuation regime.
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We have used the electric--field effect to modulate the resistivity of the surface of underdoped Sr$_{0.88}$La$_{0.12}$CuO$_{2+x}$ thin films, allowing opposite modifications of the electron and hole density in the CuO$_2$ planes, an original situation with respect to conventional chemical doping in electron-doped materials. When the Hall effect indicates a large contribution of a hole band, the electric--field effect on the normal state resistivity is however dominated by the electrons, and the superconducting transition temperature increases when carriers are transfered from holes to electrons.
We report on the spectra of point-contacts made on Sr$_{0.88}$La$_{0.12}$CuO$_2$ thin films. Besides a clear evidence for the superconducting gap, we discuss the origin of specific features, such as resistance peaks at the gap voltage and the occurrence of a two-steps resistance decrease.
High-impedance contacts made on the surface of Sr$_{0.88}$La$_{0.12}$CuO$_2$ superconducting thin films systematically display a zero-bias anomaly. We consider two-level systems (TLS) as the origin of this anomaly. We observe that the contribution of some TLS to the contact resistance is weakened by a magnetic field. We show that this could result from the increase of the TLS relaxation rate in the superconducting state, due to its ability to create pairs of quasiparticles out of the condensate, when located close to the surface of the film.
We use angle-resolved photoemission spectroscopy to study the doping evolution of infinite-layer Sr$_{1-x}$La$_{x}$CuO$_{2}$ thin films grown by molecular-beam epitaxy. At low doping, the material exhibits a dispersive lower Hubbard band typical of the superconducting cuprate parent compounds. As carriers are added to the system, a continuous evolution from charge-transfer insulator to superconductor is observed, with the initial lower Hubbard band pinned well below the Fermi level and the development of a coherent low-energy band with electron doping. This two-component spectral function emphasizes the important role that strong local correlations play even at relatively high doping levels. Electron diffraction probes reveal a ${p(2times2)}$ surface reconstruction of the material at low doping levels. Using a number of simple assumptions, we develop a model of this reconstruction based on the polar nature of the infinite-layer structure. Finally, we provide evidence for a thickness-controlled transition in ultrathin films of SrCuO$_2$ grown on nonpolar SrTiO$_3$, highlighting the diverse structural changes that can occur in polar complex oxide thin films.
Magnetic excitations in the energy range up to 100 meV are studied for over-doped La$_{2-x}$Sr$_{x}$CuO$_{4}$ with $x=0.25$ and 0.30, using time-of-flight neutron spectroscopy. Comparison of spectra integrated over the width of an antiferromagnetic Brillouin zone demonstrates that the magnetic scattering at intermediate energies, $20 lesssim omega lesssim 100$ meV, progressively decreases with over-doping. This strongly suggests that the magnetism is not related to Fermi surface nesting, but rather is associated with a decreasing volume fraction of (probably fluctuating) antiferromagnetic bubbles.
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