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Temperature dependence of uniform static magnetic susceptibility in a two-dimensional quantum Heisenberg antiferromagnetic model

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 Added by Y H Su
 Publication date 2009
  fields Physics
and research's language is English




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A perturbation spin-wave theory for the quantum Heisenberg antiferromagnets on a square lattice is proposed to calculate the uniform static magnetic susceptibility at finite temperatures, where a divergence in the previous theories due to an artificial phase transition has been removed. To the zeroth order, the main features of the uniform static susceptibility are produced: a linear temperature dependence at low temperatures and a smooth crossover in the intermediate range and the Curie law at high temperatures. When the leading corrections from the spin-wave interactions are included, the resulting spin susceptibility in the full temperature range is in agreement with the numerical quantum Monte Carlo simulations and high-temperature series expansions.



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The correlated spin dynamics and the temperature dependence of the correlation length $xi(T)$ in two-dimensional quantum ($S=1/2$) Heisenberg antiferromagnets (2DQHAF) on square lattice are discussed in the light of experimental results of proton spin lattice relaxation in copper formiate tetradeuterate (CFTD). In this compound the exchange constant is much smaller than the one in recently studied 2DQHAF, such as La$_2$CuO$_4$ and Sr$_2$CuO$_2$Cl$_2$. Thus the spin dynamics can be probed in detail over a wider temperature range. The NMR relaxation rates turn out in excellent agreement with a theoretical mode-coupling calculation. The deduced temperature behavior of $xi(T)$ is in agreement with high-temperature expansions, quantum Monte Carlo simulations and the pure quantum self-consistent harmonic approximation. Contrary to the predictions of the theories based on the Non-Linear $sigma$ Model, no evidence of crossover between different quantum regimes is observed.
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