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Register a new userEffect of a staggered spin-orbit coupling on the occurrence of a nematic phase in Sr$_3$Ru$_2$O$_7$
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Ultra-clean crystals of Sr$_3$Ru$_2$O$_7$ undergo a metamagnetic transition at low temperatures. This transition shows a strong anisotropy in the applied field direction with the critical field $H_c$ ranging from $sim 5.1$T for $Hperp c$ to $sim 8$T for $Hparallel c$. In addition, studies on ultra-pure samples revealed a bifurcation of the metamagnetic line for fields in $c$-direction and it is argued that a nematic phase emerges between the magnetization jumps. The aim of this study is to explain the field-direction anisotropy of these phenomena. Based on a microscopic tight-binding model, we introduce the metamagnetic transition by means of a van Hove singularity scenario. We show that the rotation of the O-octahedra around the c-axis expected for this material introduces a staggered spin-orbit coupling within the planes and naturally leads to an anisotropy of the magnetic response. We describe the low-temperature phase as a nematic state favored by forward scattering processes. The spin-orbit coupling shows an influence on both, the critical field $H_c$ and the occurrence of the nematic phase.
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Strong spin-orbital coupling (SOC) was found previously to lead to dramatic effects in quantum materials, such as those found in topological insulators. It was shown theoretically that local noncentrosymmetricity resulting from the rotation of RuO$_6$ octahedral in Sr$_3$Ru$_2$O$_7$ will also give rise to an effective SOCcite{SocSr327,MicroscopicnematicSr327}. In the presence of a magnetic field applied along a specific in-plane direction, the Fermi surface was predicted to undergo a reconstruction. Here we report results of our in-plane magnetoresistivity and magnetothermopower measurements on single crystals of Sr$_3$Ru$_2$O$_7$ with an electrical or a thermal current applied along specific crystalline directions and a magnetic field rotating in the $ab$ plane (Fig. 1a), showing a minimal value for field directions predicted by the local noncentrosymmetricity theory. Furthermore, the thermopower, and therefore, the electron entropy, were found to be suppressed as the field was applied perpendicular to the thermal current, which suggests that the spin and the momentum in Sr$_3$Ru$_2$O$_7$ are locked over substantial parts of the Fermi surface, likely originating from local noncentrosymmetricity as well.
We report a study of the magnetoresistivity of high purity Sr$_3$Ru$_2$O$_7$, in the vicinity of its electronic nematic phase. By employing a triple-axis (9/1/1T) vector magnet, we were able to precisely tune both the magnitude and direction of the in-plane component of the magnetic field (H$_parallel$). We report the dependence of the resistively determined anisotropy on H$_parallel$ in the phase, as well as across the wider temperature-field region. Our measurements reveal a high-temperature anisotropy which mimics the behaviour of fluctuations from the underlying quantum critical point, and suggest the existence of a more complicated phase diagram than previously reported.
We investigated Sr$_3$Ru$_2$O$_7$, a quantum critical metal that shows a metamagnetic quantum phase transition and electronic nematicity, through density functional calculations. These predict a ferromagnetic ground state in contrast to the experimentally observed paramagnetism, raising the question of competing magnetic states and associated fluctuations that may suppress magnetic order. We did a search to identify such low energy antiferromagnetically ordered metastable states. We find that the lowest energy antiferromagnetic state has a striped order. This corresponds to the E-type order that has been shown to be induced by Mn alloying. We also note significant transport anisotropy in this E-type ordered state. These results are discussed in relation to experimental observations.
X-ray magnetic critical scattering measurements and specific heat measurements were performed on the perovskite iridate Sr$_3$Ir$_2$O$_7$. We find that the magnetic interactions close to the N{e}el temperature $T_N$ = 283.4(2) K are three-dimensional. This contrasts with previous studies which suggest two-dimensional behaviour like Sr$_2$IrO$_4$. Violation of the Harris criterion ($d u>2$) means that weak disorder becomes relevant. This leads a rounding of the antiferromagnetic phase transition at $T_N$, and modifies the critical exponents relative to the clean system. Specifically, we determine that the critical behaviour of Sr$_3$Ir$_2$O$_7$ is representative of the diluted 3D Ising universality class.
We performed single electron tunneling measurements on bilayer ruthenate Sr$_3$Ru$_2$O$_7$. We observe an unusual oscillation in tunneling magnetoresistance near the metamagnetic quantum phase transition at temperatures below 7 K. The characteristic features of this oscillation suggest that it is unrelated to traditional quantum oscillations caused by orbit quantization. In addition, tunneling spectra are found to change sharply in the low bias voltage range of $V$ $<$ 2mV near the transition field. These observations reveal that the Fermi surface of Sr$_3$Ru$_2$O$_7$ changes in a surprising way as the system undergoes strong critical fluctuations.
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