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Universal decay law in charged-particle emission and exotic cluster radioactivity

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 Added by Chong Qi
 Publication date 2009
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and research's language is English




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A linear universal decay formula is presented starting from the microscopic mechanism of the charged-particle emission. It relates the half-lives of monopole radioactive decays with the $Q$-values of the outgoing particles as well as the masses and charges of the nuclei involved in the decay. This relation is found to be a generalization of the Geiger-Nuttall law in $alpha$ radioactivity and explains well all known cluster decays. Predictions on the most likely emissions of various clusters are presented.



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In the present work considering the contributions of the daughter nuclear charge and the orbital angular momentum taken away by the emitted proton, we propose a two-parameter formula of new Geiger-Nuttall law for proton radioactivity. A set of universal parameters of this law is obtained by fitting 44 experimental data of proton emitters in the ground state and isomeric state. The calculated results can reproduce the experimental data well. For a comparison, the calculations performed using other theoretical methods, such as UDLP proposed by Qi, et al. [https://journals.aps.org/prc/abstract/10.1103/PhysRevC.85.011303], the CPPM-Guo2013 analyzed by our previous work [Deng, et al., https://link.springer.com/article/10.1140/epja/i2019-12728-0] and the modified Gamow-like model proposed by us [Chen, et al., https://iopscience.iop.org/article/10.1088/1361-6471/ab1a56] are also included. Meanwhile, we extend this new Geiger-Nuttall law to predict the proton radioactivity half-lives for $51 leq Z leq 91$ nuclei, whose proton radioactivity is energetically allowed or observed but not yet quantified in NUBASE2016.
In the present work, combining with the Geiger-Nuttall law, a two-parameter empirical formula is proposed to study the two-proton (2p) radioactivity. Using this formula, the calculated 2p radioactivity half-lives are in good agreement with the experimental data as well as the calculated ones obtained by Goncalves et al: ([Phys. Lett. B 774, 14 (2017)]) using the effective liquid drop model (ELDM), Sreeja et al: ([Eur. Phys. J. A 55, 33 (2019)]) using a four-parameter empirical formula and Cui et al: ([Phys. Rev. C 101: 014301 (2020)]) using a generalized liquid drop model (GLDM). In addition, this two-parameter empirical formula is extended to predict the half-lives of 22 possible 2p radioactivity candidates, whose the 2p radioactivity released energy Q2p>0, obtained from the latest evaluated atomic mass table AME2016. The predicted results have good consistency with ones using other theoretical models such as the ELDM, GLDM and four-parameter empirical formula.
According to theory, cluster radioactivity becomes an important decay mode in superheavy nuclei. In this work, we predict that the strongly-asymmetric fission, or cluster emission, is in fact the dominant fission channel for $^{294}_{118}$Og$_{176}$, which is currently the heaviest synthetic isotope known. Our theoretical approach incorporates important features of fission dynamics, including quantum tunneling and stochastic dynamics up to scission. We show that, despite appreciable differences in static fission properties such as fission barriers and spontaneous fission lifetimes, the prediction of cluster radioactivity in $^{294}_{118}$Og$_{176}$ is robust with respect to the details of calculations, including the choice of energy density functional, collective inertia, and the strength of the dissipation term.
250 - M. Brekiesz , A. Maj , M. Kmiecik 2006
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