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Register a new userUniversal decay law in charged-particle emission and exotic cluster radioactivity
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A linear universal decay formula is presented starting from the microscopic mechanism of the charged-particle emission. It relates the half-lives of monopole radioactive decays with the $Q$-values of the outgoing particles as well as the masses and charges of the nuclei involved in the decay. This relation is found to be a generalization of the Geiger-Nuttall law in $alpha$ radioactivity and explains well all known cluster decays. Predictions on the most likely emissions of various clusters are presented.
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In the present work considering the contributions of the daughter nuclear charge and the orbital angular momentum taken away by the emitted proton, we propose a two-parameter formula of new Geiger-Nuttall law for proton radioactivity. A set of universal parameters of this law is obtained by fitting 44 experimental data of proton emitters in the ground state and isomeric state. The calculated results can reproduce the experimental data well. For a comparison, the calculations performed using other theoretical methods, such as UDLP proposed by Qi, et al. [https://journals.aps.org/prc/abstract/10.1103/PhysRevC.85.011303], the CPPM-Guo2013 analyzed by our previous work [Deng, et al., https://link.springer.com/article/10.1140/epja/i2019-12728-0] and the modified Gamow-like model proposed by us [Chen, et al., https://iopscience.iop.org/article/10.1088/1361-6471/ab1a56] are also included. Meanwhile, we extend this new Geiger-Nuttall law to predict the proton radioactivity half-lives for $51 leq Z leq 91$ nuclei, whose proton radioactivity is energetically allowed or observed but not yet quantified in NUBASE2016.
In the present work, combining with the Geiger-Nuttall law, a two-parameter empirical formula is proposed to study the two-proton (2p) radioactivity. Using this formula, the calculated 2p radioactivity half-lives are in good agreement with the experimental data as well as the calculated ones obtained by Goncalves et al: ([Phys. Lett. B 774, 14 (2017)]) using the effective liquid drop model (ELDM), Sreeja et al: ([Eur. Phys. J. A 55, 33 (2019)]) using a four-parameter empirical formula and Cui et al: ([Phys. Rev. C 101: 014301 (2020)]) using a generalized liquid drop model (GLDM). In addition, this two-parameter empirical formula is extended to predict the half-lives of 22 possible 2p radioactivity candidates, whose the 2p radioactivity released energy Q2p>0, obtained from the latest evaluated atomic mass table AME2016. The predicted results have good consistency with ones using other theoretical models such as the ELDM, GLDM and four-parameter empirical formula.
According to theory, cluster radioactivity becomes an important decay mode in superheavy nuclei. In this work, we predict that the strongly-asymmetric fission, or cluster emission, is in fact the dominant fission channel for $^{294}_{118}$Og$_{176}$, which is currently the heaviest synthetic isotope known. Our theoretical approach incorporates important features of fission dynamics, including quantum tunneling and stochastic dynamics up to scission. We show that, despite appreciable differences in static fission properties such as fission barriers and spontaneous fission lifetimes, the prediction of cluster radioactivity in $^{294}_{118}$Og$_{176}$ is robust with respect to the details of calculations, including the choice of energy density functional, collective inertia, and the strength of the dissipation term.
The 46Ti* compound nucleus, as populated by the fusion-evaporation reaction 27Al+19F at the bombarding energy of E_lab=144 MeV, has been investigated by charged particle spectroscopy using the multidetector array ICARE at the VIVITRON tandem facility of the IReS (Strasbourg). The light charged particles and high-energy gamma-rays from the GDR decay have been measured in coincidence with selected evaporation residues. The CACARIZO code, a Monte Carlo implementation of the statistical-model code CASCADE, has been used to calculate the spectral shapes of evaporated alpha-particles which are compared with the experimental coincident spectra. This comparison indicates the signature of large deformations (possibly superdeformed and hyperdeformed shapes) present in the compound nucleus decay. The occurrence of the Jacobi shape transition is also discussed in the framework of a newly developed rotating liquid drop model.
Nowadays quantum-mechanical theory allows one to reliably calculate the processes of 2p radioactivity (true three-body decays) and the corresponding energy and angular correlations up to distances of the order of 1000 fm. However, the precision of modern experiments has now become sufficient to indicate some deficiency of the predicted theoretical distributions. In this paper we discuss the extrapolation along the classical trajectories as a method to improve the convergence of the theoretical energy and angular correlations at very large distances (of the order of atomic distances), where only the long-range Coulomb forces are still operating. The precision of this approach is demonstrated using the exactly solvable semianalytical models with simplified three-body Hamiltonians. It is also demonstrated that for heavy 2p emitters, the 2p decay momentum distributions can be sensitive to the effect of the screening by atomic electrons. We compare theoretical results with available experimental data.
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