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Register a new userFluctuation-Induced Heat Release from Temperature-Quenched Nuclear Spins near a Quantum Critical Point
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At a quantum critical point (QCP) -- a zero-temperature singularity in which a line of continuous phase transition terminates -- quantum fluctuations diverge in space and time, leading to exotic phenomena that can be observed at non-zero temperatures. Using a quantum antiferromagnet, we present calorimetric evidence that nuclear spins frozen in a high-temperature metastable state by temperature quenching are annealed by quantum fluctuations near the QCP. This phenomenon, with readily detectable heat release from the nuclear spins as they are annealed, serves as an excellent marker of a quantum critical region around the QCP and provides a probe of the dynamics of the divergent quantum fluctuations.
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We present a comprehensive experimental and theoretical investigation of the thermodynamic properties: specific heat, magnetization and thermal expansion in the vicinity of the field-induced quantum critical point (QCP) around the lower critical field $H_{c1} approx 2$,T in DTN . A $T^{3/2}$ behavior in the specific heat and magnetization is observed at very low temperatures at $H=H_{c1}$ that is consistent with the universality class of Bose-Einstein condensation of magnons. The temperature dependence of the thermal expansion coefficient at $H_{c1}$ shows minor deviations from the expected $T^{1/2}$ behavior. Our experimental study is complemented by analytical calculations and Quantum Monte Carlo simulations, which reproduce nicely the measured quantities. We analyze the thermal and the magnetic Gr{u}neisen parameters that are ideal quantities to identify QCPs. Both parameters diverge at $H_{c1}$ with the expected $T^{-1}$ power law. By using the Ehrenfest relations at the second order phase transition, we are able to estimate the pressure dependencies of the characteristic temperature and field scales.
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We compute the transition temperature $T_c$ and the Ginzburg temperature $T_{rm G}$ above $T_c$ near a quantum critical point at the boundary of an ordered phase with a broken discrete symmetry in a two-dimensional metallic electron system. Our calculation is based on a renormalization group analysis of the Hertz action with a scalar order parameter. We provide analytic expressions for $T_c$ and $T_{rm G}$ as a function of the non-thermal control parameter for the quantum phase transition, including logarithmic corrections. The Ginzburg regime between $T_c$ and $T_{rm G}$ occupies a sizable part of the phase diagram.
The presence of a quantum critical point (QCP) can significantly affect the thermodynamic properties of a material at finite temperatures T. This is reflected, e.g., in the entropy landscape S(T, r) in the vicinity of a QCP, yielding particularly strong variations for varying the tuning parameter r such as pressure or magnetic field B. Here we report on the determination of the critical enhancement of $ delta S / delta B$ near a B-induced QCP via absolute measurements of the magnetocaloric effect (MCE), $(delta T / delta B)_S$, and demonstrate that the accumulation of entropy around the QCP can be used for efficient low-temperature magnetic cooling. Our proof of principle is based on measurements and theoretical calculations of the MCE and the cooling performance for a Cu$^{2+}$-containing coordination polymer, which is a very good realization of a spin-1/2 antiferromagnetic Heisenberg chain - one of the simplest quantum-critical systems.
We numerically study a model of interacting spin-$1/2$ electrons with random exchange coupling on a fully connected lattice. This model hosts a quantum critical point separating two distinct metallic phases as a function of doping: a Fermi liquid phase with a large Fermi surface volume and a low-doping phase with local moments ordering into a spin-glass. We show that this quantum critical point has non-Fermi liquid properties characterized by $T$-linear Planckian behavior, $omega/T$ scaling and slow spin dynamics of the Sachdev-Ye-Kitaev (SYK) type. The $omega/T$ scaling function associated with the electronic self-energy is found to have an intrinsic particle-hole asymmetry, a hallmark of a `skewed non-Fermi liquid.
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