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Register a new userEvidence for the existence of Kondo coupled resonant modes in heavy fermions
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Added by
Pascoal J. G. Pagliuso
Publication date
2009
fields
Physics
and research's language is
English
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Electron Spin Resonance (ESR) can microscopically probe both conduction electrons (ce) and local moment (LM) spin systems in different materials. A ce spin resonance (CESR) is observed in metallic systems based on light elements or with enhanced Pauli susceptibility. LM ESR is frequently seen in compounds with paramagnetic ions and localized d or f electrons. Here we report a remarkable and unprecedented ESR signal in the heavy fermion (HF) superconductor beta-YbAlB4[1] which behaves as a CESR at high temperatures and acquires characteristics of the Yb3+ LM ESR at low temperature. This dual behavior in same ESR spectra strikes as an in situ unique observation of the Kondo quasiparticles giving rise to a new ESR response called Kondo coupled resonant mode (KCRM). The proximity to a quantum critical point (QCP) may favor the observation of a KCRM and its dual character in beta-YbAlB4 may unveil the 4f-electrons nature at the QCP.
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Recent inelastic neutron scattering experiments in CeIn$_{3}$ and CePd$_{2}$Si$_{2}$ single crystals measured spin wave excitations at low temperatures. These two heavy fermion compounds exhibit antiferromagnetic long-range order, but a strong competition between the Ruderman-Kittel-Kasuya-Yosida(RKKY) interaction and Kondo effect is evidenced by their nearly equal Neel and Kondo temperatures. Our aim is to show how magnons such as measured in the antiferromagnetic phase of these Ce compounds, can be described with a microscopic Heisenberg-Kondo model introduced by J.R.Iglesias, C.Lacroix and B.Coqblin, used before for studies of the non-magnetic phase. The model includes the correlated Ce-$4 f$ electrons hybridized with the conduction band, where we also allow for correlations, and we consider competing RKKY (Heisenberg-like $J_{H} $) and Kondo ($J_{K}$) antiferromagnetic couplings. Carrying on a series of unitary transformations, we perturbatively derive a second-order effective Hamiltonian which, projected onto the antiferromagnetic electron ground state, describes the spin wave excitations, renormalized by their interaction with correlated itinerant electrons. We numerically study how the different parameters of the model influence the renormalization of the magnons, yielding useful information for the analysis of inelastic neutron scattering experiments in antiferromagnetic heavy fermion compounds. We also compare our results with the available experimental data, finding good agreement with the spin wave measurements in cubic CeIn$_3$.
Resolving the heavy fermion band in the conduction electron momentum resolved spectral function of the Kondo lattice model is challenging since, in the weak coupling limit, its spectral weight is exponentially small. In this article we consider a composite fermion operator, consisting of a conduction electron dressed by spin fluctuations that shares the same quantum numbers as the electron operator. Using approximation free auxiliary field quantum Monte Carlo simulations we show that for the SU(2) spin-symmetric model on the square lattice at half filling, the composite fermion acts as a magnifying glass for the heavy fermion band. In comparison to the conduction electron residue that scales as $e^{-W/J_k}$ with $W$ the bandwidth and $J_k$ the Kondo coupling, the residue of the composite fermion tracks $J_k$. This result holds down to $J_k/W = 0.05$, and confirms the point of view that magnetic ordering, present below $J_k/W = 0.18$, does not destroy the heavy quasiparticle. We furthermore investigate the spectral function of the composite fermion in the ground state and at finite temperatures, for SU($N$) generalizations of the Kondo lattice model, as well as for ferromagnetic Kondo couplings, and compare our results to analytical calculations in the limit of high temperatures, large-$N$, large-$S$, and large $J_k$. Based on these calculations, we conjecture that the composite fermion operator provides a unique tool to study the destruction of the heavy fermion quasiparticle in Kondo breakdown transitions. The relation of our results to scanning tunneling spectroscopy and photoemission experiments is discussed.
One of the challenges in strongly correlated electron systems, is to understand the anomalous electronic behavior that develops at an antiferromagnetic quantum critical point (QCP), a phenomenon that has been extensively studied in heavy fermion materials. Current theories have focused on the critical spin fluctuations and associated break-down of the Kondo effect. Here we argue that the abrupt change in Fermi surface volume that accompanies heavy fermion criticality leads to critical charge fluctuations. Using a model one dimensional Kondo lattice in which each moment is connected to a separate conduction bath, we show a Kondo breakdown transition develops between a heavy Fermi liquid and a gapped spin liquid via a QCP with omega/T scaling, which features a critical charge mode directly associated with the break-up of Kondo singlets. We discuss the possible implications of this emergent charge mode for experiment.
Recent inelastic neutron scattering experiments in CeIn3 and CePd2Si2 single crystals, measured spin wave excitations at low temperatures. These two heavy fermion compounds exhibit antiferromagnetic long-range order, but a strong competition between the Ruderman-Kittel-Kasuya-Yosida(RKKY) interaction and Kondo effect is evidenced by their nearly equal Neel and Kondo temperatures. Our aim is to show how magnons such as measured in the antiferromagnetic phase of these Ce compounds, can be described with a microscopic Heisenberg-Kondo model as introduced by J.R.Iglesias, C.Lacroix and B.Coqblin, used before for studies of the non-magnetic phase. The model includes the correlated Ce-4f electrons hybridized with the conduction band, and we consider competing RKKY (Heisenberg-like J_{H}) and Kondo (J_{K}) antiferromagnetic couplings. Carrying on a series of unitary transformations, we perturbatively derive a second-order effective Hamiltonian which, projected onto the antiferromagnetic electron ground state, describes the spin wave excitations, renormalized by their interaction with correlated itinerant electrons. We numerically study how the different parameters of the model influence the renormalization of the magnons, yielding useful information for the analysis of inelastic neutron scattering experiments in antiferromagnetic heavy fermion compounds. We also compare our results with available experimental data, finding good agreement with the spin wave measurements in cubic CeIn3.
Resonant X-ray scattering (RXS) has recently become an increasingly important tool for the study of ordering phenomena in correlated electron systems. Yet, the interpretation of the RXS experiments remains theoretically challenging due to the complexity of the RXS cross-section. Central to this debate is the recent proposal that impurity-induced Friedel oscillations, akin to quasiparticle interference signals observed with the scanning tunneling microscope (STM), can lead to scattering peaks in the RXS experiments. The possibility that quasiparticle properties can be probed in RXS measurements opens up a new avenue to study the bulk band structure of materials with the orbital and element selectivity provided by RXS. Here, we test these ideas by combining RXS and STM measurements of the heavy fermion compound CeMIn$_5$ (M = Co, Rh). Temperature and doping dependent RXS measurements at the Ce-M$_4$ edge show a broad scattering enhancement that correlates with the appearance of heavy f-electron bands in these compounds. The scattering enhancement is consistent with the measured quasiparticle interference signal in the STM measurements, indicating that quasiparticle interference can be probed through the momentum distribution of RXS signals. Overall, our experiments demonstrate new opportunities for studies of correlated electronic systems using the RXS technique.
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