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Register a new userThe cleavage surface of the BaFe_(2-x)Co_(x)As_(2) and Fe_(y)Se_(1-x)Te_(x) superconductors: from diversity to simplicity
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We elucidate the termination surface of cleaved single crystals of the BaFe_(2-x)Co_(x)As_(2) and Fe_(y)Se_(1-x)Te_(x) families of the high temperature iron based superconductors. By combining scanning tunneling microscopic data with low energy electron diffraction we prove that the termination layer of the Ba122 systems is a remnant of the Ba layer, which exhibits a complex diversity of ordered and disordered structures. The observed surface topographies and their accompanying superstructure reflections in electron diffraction depend on the cleavage temperature. In stark contrast, Fe_(y)Se_(1-x)Te_(x) possesses only a single termination structure - that of the tetragonally ordered Se_(1-x)Te_(x) layer.
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Doping dependence of the superconducting state structure and spin-fluctuation pairing mechanism in the $Ba(Fe_{1-x}Co_{x})_{2}As_{2}$ family is studied. BCS-like analysis of experimental data shows that in the overdoped regime, away from the AFM transition, the spin-fluctuation interaction between the electron and hole gaps is weak, and $Ba(Fe_{1-x}Co_{x})_{2}As_{2}$ is characterized by three essentially different gaps. In the three-gap state an anisotropic (nodeless) electron gap $Delta_e (x, phi)$ has an intermediate value between the dominant inner $Delta_{2h}(x)$ and outer $Delta_{1h}(x)$ hole gaps. Close to the AFM transition the electron gap $Delta_e (x, phi)$ increases sharply and becomes closer in magnitude to the dominant inner hole gap $Delta_{2h}(x)$. The same two-gap state with close electron and inner hole gaps $Delta_{2h}(x) approx Delta_e (x, phi)$ is also preserved in the phase of coexisting antiferromagnetism and superconductivity. The doping dependence of the electron gap $Delta_e (x, phi)$ is associated with the strong doping dependence of the spin-fluctuation interaction in the AFM transition region. In contrast to the electron gap $Delta_e (x, phi)$, the doping dependence of the hole gaps $Delta_{1,2h}(x)$ and the critical temperature $T_{c}(x)$, both before and after the AFM transition, are associated with a change of the density of states $gamma_{nh}(x)$ and the intraband electron-phonon interaction in the hole bands. The non-phonon spin-fluctuation interaction in the hole bands in the entire Co concentration range is small compared with the intraband electron-phonon interaction and is not dominant in the $Ba(Fe_{1-x}Co_{x})_{2}As_{2}$ family.
We use scanning SQUID microscopy to investigate the behavior of vortices in the presence of twin boundaries in the pnictide superconductor Ba(Fe1-xCox)2As2. We show that the vortices avoid pinning on twin boundaries. Individual vortices move in a preferential way when manipulated with the SQUID: they tend to not cross a twin boundary, but rather to move parallel to it. This behavior can be explained by the observation of enhanced superfluid density on twin boundaries in Ba(Fe1-xCox)2As2. The observed repulsion from twin boundaries may be a mechanism for enhanced critical currents observed in twinned samples in pnictides and other superconductors.
The magnetic and superconducting properties of a series of underdoped $Ba_{1-x}Na_{x}Fe_{2}As_{2}$ (BNFA) single crystals with $0.19 leq xleq 0.34$ has been investigated with the complementary muon-spin-rotation ($mu$SR) and infrared spectroscopy techniques. The focus has been on the different antiferromagnetic states in the underdoped regime and their competition with superconductivity, especially for the ones with a tetragonal crystal structure and a so-called double-$Q$ magnetic order. Besides the collinear state with a spatially inhomogeneous spin-charge-density wave (i-SCDW) order at $x=0.24$ and $0.26$, that was previously identified in BNFA, we obtained evidence for an orthomagnetic state with a hedgehog-type spin vortex crystal (SVC) structure at $x=0.32$ and $0.34$. Whereas in the former i-SCDW state the infrared spectra show no sign of a superconducting response down to the lowest measured temperature of about 10K, in the SVC state there is a strong superconducting response similar to the one at optimum doping. The magnetic order is strongly suppressed here in the superconducting state and at $x=0.34$ there is even a partial re-entrance into a paramagnetic state at $T<<T_c$.
We develop a local spin model to explain the rich magnetic structures in the iron-based superconductors $Fe_{1+y}Te_{1-x}Se_x$. We show that our model exhibits both commensurate antiferromagnetic and incommensurate magnetic order along the crystal a-axis. The transition from the commensurate to the incommensurate phase is induced when the concentration of excess $Fe$ atoms is larger than a critical value. Experimentally measurable spin-wave features are calculated, and the mean-field phase diagram of the model is obtained. Our model also suggests the existence of a large quantum critical region due to strong spin frustration upon increasing $Se$ concentration.
The local structure and electronic properties of Rb$_{1-x}$Fe$_{2-y}$Se$_2$ are investigated by means of site selective polarized x-ray absorption spectroscopy at the iron and selenium K-edges as a function of pressure. A combination of dispersive geometry and novel nanodiamond anvil pressure-cell has permitted to reveal a step-like decrease in the Fe-Se bond distance at $psimeq11$ GPa. The position of the Fe K-edge pre-peak, which is directly related to the position of the chemical potential, remains nearly constant until $sim6$ GPa, followed by an increase until $psimeq 11$ GPa. Here, as in the local structure, a step-like decrease of the chemical potential is seen. Thus, the present results provide compelling evidence that the origin of the reemerging superconductivity in $A_{1-x}$Fe$_{2-y}$Se$_2$ in vicinity of a quantum critical transition is caused mainly by the changes in the electronic structure.
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