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Register a new userResonant Magnetic X-ray Diffraction Study on the Triangular Lattice Antiferromagnet GdPd2Al3
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Resonant magnetic x-ray diffraction experiments were carried out on the stacked triangular lattice antiferromagnet GdPd2Al3. The experiments revealed an expected initial collinear c-axis order at TN1 followed by an additional in-plane order at TN2, while at the same time we found that the ground state is a helically ordered state of a very long incommensurate period of approximately 700A. The distribution of K-domains was highly anisotropic, and the domain with the modulation vector normal to the surface of the crystal was ascendant. Low-field magnetization is discussed on the basis of the observed incommensurate magnetic structure.
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Resonant x-ray scattering is performed near the Mn K-absorption edge for an epitaxial thin film of BiMnO3. The azimuthal angle dependence of the resonant (003) peak (in monoclinic indices) is measured with different photon polarizations; for the $sigmatopi$ channel a 3-fold symmetric oscillation is observed in the intensity variation, while the $sigmatosigma$ scattering intensity remains constant. These features are accounted for in terms of the peculiar ordering of the manganese 3d orbitals in BiMnO3. It is demonstrated that the resonant peak persists up to 770 K with an anomaly around 440 K; these high and low temperatures coincide with the structural transition temperatures, seen in bulk, with and without a symmetry change, respectively. A possible relationship of the orbital order with the ferroelectricity of the system is discussed.
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We performed neutron single crystal and synchrotron X-ray powder diffraction experiments in order to investigate the magnetic and crystal structures of the conductive layered triangular-lattice antiferromagnet PdCrO2 with a putative spin chirality, which contributes to an unconventional anomalous Hall effect. We revealed that the ground-state magnetic structure is a commensurate and nearly-coplanar 120-degrees spin structure. The 120-degrees plane in different Cr layers seem to tilt with one another, leading to a small noncoplanarity. Such a small but finite non-coplanar stacking of the 120-degrees planes gives rise to a finite scalar spin chirality, which may be responsible for the unconventional nature of the Hall effect of PdCrO2.
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