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Register a new userLaser microfluidics: fluid actuation by light
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The development of microfluidic devices is still hindered by the lack of robust fundamental building blocks that constitute any fluidic system. An attractive approach is optical actuation because light field interaction is contactless and dynamically reconfigurable, and solutions have been anticipated through the use of optical forces to manipulate microparticles in flows. Following the concept of an optical chip advanced from the optical actuation of suspensions, we propose in this survey new routes to extend this concept to microfluidic two-phase flows. First, we investigate the destabilization of fluid interfaces by the optical radiation pressure and the formation of liquid jets. We analyze the droplet shedding from the jet tip and the continuous transport in laser-sustained liquid channels. In the second part, we investigate a dissipative light-flow interaction mechanism consisting in heating locally two immiscible fluids to produce thermocapillary stresses along their interface. This opto-capillary coupling is implemented in adequate microchannel geometries to manipulate two-phase flows and propose a contactless optical toolbox including valves, droplet sorters and switches, droplet dividers or droplet mergers. Finally, we discuss radiation pressure and opto-capillary effects in the context of the optical chip where flows, channels and operating functions would all be performed optically on the same device.
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We unveil the generation of universal morphologies of fluid interfaces by radiation pressure whatever is the nature of the wave, acoustic or optical. Experimental observations reveal interface deformations endowed with step-like features that are shown to result from the interplay between the wave propagation and the shape of the interface. The results are supported by numerical simulations and a quantitative interpretation based on the waveguiding properties of the field is provided.
The deformation of a fluid-fluid interface due to the thermocapillary stress induced by a continuous Gaussian laser wave is investigated analytically. We show that the direction of deformation of the liquid interface strongly depends on the viscosities and the thicknesses of the involved liquid layers. We first investigate the case of an interface separating two different liquid layers while a second part is dedicated to a thin film squeezed by two external layers of same liquid. These results are predictive for applications fields where localized thermocapillary stresses are used to produce flows or to deform interfaces in presence of confinement, such as optofluidics.
When a surfactant-stabilised oil droplet with an ultralow interfacial tension is trapped in the focus of two laser beams and pulled apart (by moving the laser beams) a configuration of two droplets connected by a thin tether of oil results. The tether radius depends on the ratio of the bending modulus to the renormalized interfacial tension, which takes into account the spontaneous curvature of the interface. The force exerted by the tether on the droplets is shown to be asymmetric with respect to the phase inversion temperature of the emulsion, in agreement with experiment. Fluid can be pumped from one droplet to the other via the tether by increasing the optical pressure on one droplet. The flow is a combination of Poiseuille flow within the thread of oil and the external flow around a rigid cylinder, with the surface velocity determined by tangential stress balance. For typical viscosities of oils and the continuous aqueous medium, flow is predominantly in the external medium. The normal stress balance leads to a variation in the radius of the thread with distance. The radius is shown to decrease approximately linearly with a slope proportional to the volumetric flow rate through the tether. For a tether of a given length, there is therefore an upper limit to the flow rate that can be generated by pumping with optical traps.
Droplet-based high throughput biomolecular screening and combinatorial synthesis entail a viable indexing strategy to be developed for the identification of each micro-reactor. Here, we propose a novel indexing scheme based on the generation of droplet sequences on demand to form unique encoding droplet chains in fluidic networks. These codes are represented by multiunit and multilevel droplets packages, with each code unit possessing several distinct signal levels, potentially allowing large encoding capacity. For proof of concept, we use magnetic nanoparticles as the encoding material and a giant magnetoresistance (GMR) sensor-based active sorting system supplemented with an optical detector to generate and decode the sequence of one exemplar sample droplet reactor and a 4-unit quaternary magnetic code. The indexing capacity offered by 4-unit multilevel codes with this indexing strategy is estimated to exceed 104, which holds great promise for large-scale droplet-based screening and synthesis.
Staggered and linear multi-particle trains constitute characteristic structures in inertial microfluidics. Using lattice-Boltzmann simulations, we investigate their properties and stability, when flowing through microfluidic channels. We confirm the stability of cross-streamline pairs by showing how they contract or expand to their equilibrium axial distance. In contrast, same-streamline pairs quickly expand to a characteristic separation but even at long times slowly drift apart. We reproduce the distribution of particle distances with its characteristic peak as measured in experiments. Staggered multi-particle trains initialized with an axial particle spacing larger than the equilibrium distance contract non-uniformly due to collective drag reduction. Linear particle trains, similar to pairs, rapidly expand towards a value about twice the equilibrium distance of staggered trains and then very slowly drift apart non-uniformly. Again, we reproduce the statistics of particle distances and the characteristic peak observed in experiments. Finally, we thoroughly analyze the damped displacement pulse traveling as a microfluidic phonon through a staggered train and show how a defect strongly damps its propagation.
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