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Quantum oscillations in the anomalous phase in Sr3Ru2O7

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 Publication date 2009
  fields Physics
and research's language is English




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We report measurements of quantum oscillations detected in the putative nematic phase of Sr3Ru2O7. Significant improvements in sample purity enabled the resolution of small amplitude dHvA oscillations between two first order metamagnetic transitions delimiting the phase. Two distinct frequencies were observed, and their amplitudes follow the normal Lifshitz-Kosevich profile. The Fermi surface sheets seem to correspond to a subset of those detected outside the phase. Variations of the dHvA frequencies are explained in terms of a chemical potential shift produced by reaching a peak in the density of states, and an anomalous field dependence of the oscillatory amplitude provides information on domains.



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We report detailed investigation of quantum oscillations in Sr3Ru2O7, observed inductively (the de Haas-van Alphen effect) and thermally (the magnetocaloric effect). Working at fields from 3 T to 18 T allowed us to straddle the metamagnetic transition region and probe the low- and high-field Fermi liquids. The observed frequencies are strongly field-dependent in the vicinity of the metamagnetic transition, and there is evidence for magnetic breakdown. We also present the results of a comprehensive rotation study. The most surprising result concerns the field dependence of the measured quasiparticle masses. Contrary to conclusions previously drawn by some of us as a result of a study performed with a much poorer signal to noise ratio, none of the five Fermi surface branches for which we have good field-dependent data gives evidence for a strong field dependence of the mass. The implications of these experimental findings are discussed.
The behaviour of matter near zero temperature continuous phase transitions, or quantum critical points (QCPs) is a central topic of study in condensed matter physics. In fermionic systems, fundamental questions remain unanswered: the nature of the quantum critical regime is unclear because of the apparent breakdown of the concept of the quasiparticle, a cornerstone of existing theories of strongly interacting metals. Even less is known experimentally about the formation of ordered phases from such a quantum critical soup. Here, we report a study of the specific heat across the phase diagram of the model system Sr3Ru2O7, which features an anomalous phase whose transport properties are consistent with those of an electronic nematic. We show that this phase, which exists at low temperatures in a narrow range of magnetic fields, forms directly from a quantum critical state, and contains more entropy than mean-field calculations predict. Our results suggest that this extra entropy is due to remnant degrees of freedom from the highly entropic state above T_c. The associated quantum critical point, which is concealed by the nematic phase, separates two Fermi liquids, neither of which has an identifiable spontaneously broken symmetry, but which likely differ in the topology of their Fermi surfaces.
Shubnikov--de Haas (SdH) and Hall-effect measurements of CeBiPt and LaBiPt reveal the presence of simple and very small Fermi surfaces with hole-like charge carriers for both semimetals. In the magnetic material, CeBiPt, we observe a strong temperature dependence of the SdH frequency. This highly unusual effect might be connected with an internal exchange field within the material and a strongly spin-dependent scattering of the charge carriers.
The quantum de Haas van Alphen (dHvA) and Shubnikov de Haas (SdH) oscillations measured in graphite were decomposed by pass-band filtering onto contributions from three different groups of carriers. We develop the two-dimensional phase analysis method which allows to identify these carriers as (i) minority holes having two-dimensional (2D) parabolic massive spectrum, (ii) majority electrons, also massive but with intermediate 2D-3D spectrum, and (iii) majority holes with 2D Dirac-like spectrum which seems to be responsible for the unusual strongly-correlated electronic phenomena in graphite.
Thermal conductivity of Sr3Ru2O7 was measured down to 40 mK and at magnetic fields through the quantum critical endpoint at H_c = 7.85 T. A peak in the electrical resistivity as a function of field was mimicked by the thermal resistivity. In the limit as T -> 0 K we find that the Wiedemann-Franz law is satisfied to within 5% at all fields, implying that there is no breakdown of the electron despite the destruction of the Fermi liquid state at quantum criticality. A significant change in disorder (from $rho_0$(H=0T) = 2.1 $muOmega$ cm to 0.5 $muOmega$ cm) does not influence our conclusions. At finite temperatures, the temperature dependence of the Lorenz number is consistent with ferromagnetic fluctuations causing the non-Fermi liquid behavior as one would expect at a metamagnetic quantum critical endpoint.
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