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Register a new userSpin canting in a Dy-based Single-Chain Magnet with dominant next-nearest neighbor antiferromagnetic interactions
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We investigate theoretically and experimentally the static magnetic properties of single crystals of the molecular-based Single-Chain Magnet (SCM) of formula [Dy(hfac)$_{3}$NIT(C$_{6}$H$_{4}$OPh)]$_{infty}$ comprising alternating Dy$^{3+}$ and organic radicals. A peculiar inversion between maxima and minima in the angular dependence of the magnetic molar susceptibility $chi_{M}$ occurs on increasing temperature. Using information regarding the monomeric building block as well as an {it ab initio} estimation of the magnetic anisotropy of the Dy$^{3+}$ ion, this anisotropy-inversion phenomenon can be assigned to weak one-dimensional ferromagnetism along the chain axis. This indicates that antiferromagnetic next-nearest-neighbor interactions between Dy$^{3+}$ ions dominate, despite the large Dy-Dy separation, over the nearest-neighbor interactions between the radicals and the Dy$^{3+}$ ions. Measurements of the field dependence of the magnetization, both along and perpendicularly to the chain, and of the angular dependence of $chi_{M}$ in a strong magnetic field confirm such an interpretation. Transfer matrix simulations of the experimental measurements are performed using a classical one-dimensional spin model with antiferromagnetic Heisenberg exchange interaction and non-collinear uniaxial single-ion anisotropies favoring a canted antiferromagnetic spin arrangement, with a net magnetic moment along the chain axis. The fine agreement obtained with experimental data provides estimates of the Hamiltonian parameters, essential for further study of the dynamics of rare-earths based molecular chains.
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We calculate the quantum phase diagram of the {it XXZ} chain with nearest-neighbor (NN) $J_{1}$ and next-NN exchange $J_{2}$ with anisotropies $Delta_{1}$ and $Delta_{2}$ respectively. In particular we consider the case $Delta_{1}=-Delta_{2}$ to interpolate between the {it XX} chain ($% Delta_{i}=0$) and the isotropic model with ferromagnetic $J_{2}$. For $% Delta_{1}<-1$, a ferromagnetic and two antiferromagnetic phases exist. For $| Delta_{i}| <1$, the boundary between the dimer and spin fluid phases is determined by the method of crossing of excitation spectra. For large $J_{2}/J_{1}$, this method seems to indicate the existence of a second spin fluid critical phase. However, an analysis of the spin stiffness and magnetic susceptibility for $Delta_{1}=Delta_{2}=1$ suggest that a small gap is present.
We implement a new and accurate numerical entropic scheme to investigate the first-order transition features of the triangular Ising model with nearest-neighbor ($J_{nn}$) and next-nearest-neighbor ($J_{nnn}$) antiferromagnetic interactions in ratio $R=J_{nn}/J_{nnn}=1$. Important aspects of the existing theories of first-order transitions are briefly reviewed, tested on this model, and compared with previous work on the Potts model. Using lattices with linear sizes $L=30,40,...,100,120,140,160,200,240,360$ and 480 we estimate the thermal characteristics of the present weak first-order transition. Our results improve the original estimates of Rastelli et al. and verify all the generally accepted predictions of the finite-size scaling theory of first-order transitions, including transition point shifts, thermal, and magnetic anomalies. However, two of our findings are not compatible with current phenomenological expectations. The behavior of transition points, derived from the number-of-phases parameter, is not in accordance with the theoretically conjectured exponentially small shift behavior and the well-known double Gaussian approximation does not correctly describe higher correction terms of the energy cumulants. It is argued that this discrepancy has its origin in the commonly neglected contributions from domain wall corrections.
Low-energy magnetic excitations in the spin-1/2 chain compound (C$_6$H$_9$N$_2$)CuCl$_3$ [known as (6MAP)CuCl$_3$] are probed by means of tunable-frequency electron spin resonance. Two modes with asymmetric (with respect to the $h u=gmu_B B$ line) frequency-field dependences are resolved, illuminating the striking incompatibility with a simple uniform $S=frac{1}{2}$ Heisenberg chain model. The unusual ESR spectrum is explained in terms of the recently developed theory for spin-1/2 chains, suggesting the important role of next-nearest-neighbor interactions in this compound. Our conclusion is supported by model calculations for the magnetic susceptibility of (6MAP)CuCl$_3$, revealing a good qualitative agreement with experiment.
A chiral $p_x+ip_y$ superconductor on a square lattice with nearest and next-nearest hopping and pairing terms is considered. Gap closures, as various parameters of the system are varied, are found analytically and used to identify the topological phases. The phases are characterized by Chern numbers (ranging from -3 to 3), and (numerically) by response to introduction of weak disorder, edges, and magnetic fields in an extreme type-II limit, focusing on the low-energy modes (which presumably become zero-energy Majorana modes for large lattices and separations). Several phases are found, including a phase with Chern number 3 that cannot be thought of in terms of a single range of interaction, and phase with Chern number 2 that may host an additional, disorder resistant, Majorana mode. The energies of the vortex quasiparticle modes were found to oscillate as vortex position varied. The spatial length scale of these oscillations was found for various points in the Chern number 3 phase which increased as criticality was approached.
The evolution of entanglement in a 3-spin chain with nearest-neighbor Heisenberg-XY interactions for different initial states is investigated here. In an NMR experimental implementation, we generate multipartite entangled states starting from initial separable pseudo-pure states by simulating nearest-neighbor XY interactions in a 3-spin linear chain of nuclear spin qubits. For simulating XY interactions, we follow algebraic method of Zhang et al. [Phys. Rev. A 72, 012331 (2005)]. Bell state between end qubits has been generated by using only the unitary evolution of the XY Hamiltonian. For generating W-state and GHZ-state a single qubit rotation is applied on second and all the three qubits respectively after the unitary evolution of the XY Hamiltonian.
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