No Arabic abstract
Low-energy magnetic excitations in the spin-1/2 chain compound (C$_6$H$_9$N$_2$)CuCl$_3$ [known as (6MAP)CuCl$_3$] are probed by means of tunable-frequency electron spin resonance. Two modes with asymmetric (with respect to the $h u=gmu_B B$ line) frequency-field dependences are resolved, illuminating the striking incompatibility with a simple uniform $S=frac{1}{2}$ Heisenberg chain model. The unusual ESR spectrum is explained in terms of the recently developed theory for spin-1/2 chains, suggesting the important role of next-nearest-neighbor interactions in this compound. Our conclusion is supported by model calculations for the magnetic susceptibility of (6MAP)CuCl$_3$, revealing a good qualitative agreement with experiment.
The purpose of this note is to connect early work on thermal transport in spin-1/2 Heisenberg chains with uniaxial exchange anisotropy and nearest-neighbor interactions that was based on a moment analysis of the Fourier transform of the energy density correlation function with subsequent studies that make use of thermal current correlation functions.
The magnetic susceptibility $chi(T)$ of spin-1/2 chains is widely used to quantify exchange interactions, even though $chi(T)$ is similar for different combinations of ferromagnetic $J_1$ between first neighbors and antiferromagnetic $J_2$ between second neighbors. We point out that the spin specific heat $C(T)$ directly determines the ratio $alpha = J_2/|J_1|$ of competing interactions. The $J_1-J_2$ model is used to fit the isothermal magnetization $M(T,H)$ and $C(T,H)$ of spin-1/2 Cu(II) chains in LiCuSbO$_4$. By fixing $alpha$, $C(T)$ resolves the offsetting $J_1$, $alpha$ combinations obtained from $M(T,H)$ in cuprates with frustrated spin chains.
We describe why Ising spin chains with competing interactions in $rm SrHo_2O_4$ segregate into ordered and disordered ensembles at low temperatures ($T$). Using elastic neutron scattering, magnetization, and specific heat measurements, the two distinct spin chains are inferred to have Neel ($uparrowdownarrowuparrowdownarrow$) and double-Neel ($uparrowuparrowdownarrowdownarrow$) ground states respectively. Below $T_mathrm{N}=0.68(2)$~K, the Neel chains develop three dimensional (3D) long range order (LRO), which arrests further thermal equilibration of the double-Neel chains so they remain in a disordered incommensurate state for $T$ below $T_mathrm{S}= 0.52(2)$~K. $rm SrHo_2O_4$ distills an important feature of incommensurate low dimensional magnetism: kinetically trapped topological defects in a quasi$-d-$dimensional spin system can preclude order in $d+1$ dimensions.
The spin-$frac{1}{2}$ kagome antiferromagnet is an archetypal frustrated system predicted to host a variety of exotic magnetic states. We show using neutron scattering measurements that deuterated vesignieite BaCu$_{3}$V$_{2}$O$_{8}$(OD)$_{2}$, a fully stoichiometric $S=1/2$ kagome magnet with $<$1% lattice distortion, orders magnetically at $T_{mathrm{N}}=9$K into a multi-k coplanar variant of the predicted triple-k octahedral structure. We find this structure is stabilized by a dominant antiferromagnetic 3$^{mathrm{rd}}$-neighbor exchange $J_3$ with minor 1$^{mathrm{st}}$- or 2$^{mathrm{nd}}$--neighbour exchange. The spin-wave spectrum is well described by a $J_3$-only model including a tiny symmetric exchange anisotropy.
We investigate the phase diagrams of a one-dimensional lattice model of fermions and of a spin chain with interactions extending up to next-nearest neighbour range. In particular, we investigate the appearance of regions with dominant pairing physics in the presence of nearest-neighbour and next-nearest-neighbour interactions. Our analysis is based on analytical calculations in the classical limit, bosonization techniques and large-scale density-matrix renormalization group numerical simulations. The phase diagram, which is investigated in all relevant filling regimes, displays a remarkably rich collection of phases, including Luttinger liquids, phase separation, charge-density waves, bond-order phases, and exotic cluster Luttinger liquids with paired particles. In relation with recent studies, we show several emergent transition lines with a central charge $c = 3/2$ between the Luttinger-liquid and the cluster Luttinger liquid phases. These results could be experimentally investigated using highly-tunable quantum simulators.