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Register a new userNano-scale brushes: How to build a smart surface coating
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Via computer simulations, we demonstrate how a densely grafted layer of polymers, a {it brush}, could be turned into an efficient switch through chemical modification of some of its end-monomers. In this way, a surface coating with reversibly switchable properties can be constructed. We analyze the fundamental physical principle behind its function, a recently discovered surface instability, and demonstrate that the combination of a high grafting density, an inflated end-group size and a high degree of monodispersity are conditions for an optimal functionality of the switch.
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In recent years there have been a number of proposals to utilize the specificity of DNA based interactions for potential applications in nanoscience. One interesting direction is the self-assembly of micro- and nanoparticle clusters using DNA scaffolds. In this letter we consider a DNA scaffold method to self-assemble clusters of colored particles. Stable clusters of microspheres have recently been produced by an entirely different method. Our DNA based approach self-assembles clusters with additional degrees of freedom associated with particle permutation. We demonstrate that in the non-equilibrium regime of irreversible binding the self-assembly process is experimentally feasible. These color degrees of freedom may allow for more diverse intercluster interactions essential for hierarchical self-assembly of larger structures.
The world is changing at an ever-increasing pace. And it has changed in a much more fundamental way than one would think, primarily because it has become more connected and interdependent than in our entire history. Every new product, every new invention can be combined with those that existed before, thereby creating an explosion of complexity: structural complexity, dynamic complexity, functional complexity, and algorithmic complexity. How to respond to this challenge? And what are the costs?
Given two copies of any quantum mechanical system, one may want to prepare them in the thermofield double state for the purpose of studying thermal physics or black holes. However, the thermofield double is a unique entangled pure state and may be difficult to prepare. We propose a local interacting Hamiltonian for the combined system whose ground state is approximately the thermofield double. The energy gap for this Hamiltonian is of order the temperature. Our construction works for any quantum system satisfying the Eigenvalue Thermalization Hypothesis.
Cosmic voids provide a powerful probe of the origin and evolution of structures in the Universe because their dynamics can remain near-linear to the present day. As a result they have the potential to connect large scale structure at late times to early-Universe physics. Existing watershed-based algorithms, however, define voids in terms of their morphological properties at low redshift. The degree to which the resulting regions exhibit linear dynamics is consequently uncertain, and there is no direct connection to their evolution from the initial density field. A recent void definition addresses these issues by considering anti-halos. This approach consists of inverting the initial conditions of an $N$-body simulation to swap overdensities and underdensities. After evolving the pair of initial conditions, anti-halos are defined by the particles within the inverted simulation that are inside halos in the original (uninverted) simulation. In this work, we quantify the degree of non-linearity of both anti-halos and watershed voids using the Zeldovich approximation. We find that non-linearities are introduced by voids with radii less than $5,mathrm{Mpc},h^{-1}$, and that both anti-halos and watershed voids can be made into highly linear sets by removing these voids.
The structure of spherical micelles of the diblock copolymer poly(styrene-block-acrylic acid) in water was investigated with small angle neutron scattering (SANS) and contrast matching. We have monitored inter-micelle correlation and the extension of the polyelectrolyte chains in the coronal layer through the overlap concentration. Irrespective of ionic strength, the corona shrinks with increasing packing fraction. Furthermore, at high charge and minimal screening conditions, the corona layers interpenetrate once the volume fraction exceeds the critical value 0.53.
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