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Register a new userSlow Relaxation and Equilibrium Dynamics in a 2 D Coulomb Glass: Demonstration of Stretched Exponential Energy Correlations
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We have simulated energy relaxation and equilibrium dynamics in Coulomb Glasses using the random energy lattice model. We show that in a temperature range where the Coulomb Gap is already well developed, (T=0.03-0.1) the system still relaxes to an equilibrium behavior within the simulation time scale. For all temperatures T, the relaxation is slower than exponential. Analyzing the energy correlations of the system at equilibrium, we find a stretched exponential behavior. We define a time tau_gamma from these stretched exponential correlations, and show that this time corresponds well with the time required to reach equilibrium. From our data it is not possible to determine whether tau_gamma diverges at any finite temperature, indicating a glass transition, or whether this divergence happens at zero temperature. While the time dependence of the system energy can be well fitted by a random walker in a harmonic potential for high temperatures (T=10), this simple model fails to describe the long time scales observed at lower temperatures. Instead we present an interpretation of the configuration space as a structure with fractal properties, and the time evolution as a random walk on this fractal-like structure.
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The relaxation of the specific heat and the entropy to their equilibrium values is investigated numerically for the three-dimensional Coulomb glass at very low temperatures. The long time relaxation follows a stretched exponential function, $f(t)=f_0exp[-(t/tau)^beta]$, with the exponent $beta$ increasing with the temperature. The relaxation time follows an Arrhenius behavior divergence when $Tto 0$. A relation between the specific heat and the entropy in the long time regime is found.
We propose an atomistic model for correlated particle dynamics in liquids and glasses predicting both slow stretched-exponential relaxation (SER) and fast compressed-exponential relaxation (CER). The model is based on the key concept of elastically interacting local relaxation events. SER is related to slowing down of dynamics of local relaxation events as a result of this interaction, whereas CER is related to the avalanche-like dynamics in the low-temperature glass state. The model predicts temperature dependence of SER and CER seen experimentally and recovers the simple, Debye, exponential decay at high temperature. Finally, we reproduce SER to CER crossover across the glass transition recently observed in metallic glasses.
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This paper is concerned with the connection between the properties of dielectric relaxation and ac (alternating-current) conduction in disordered dielectrics. The discussion is divided between the classical linear-response theory and a self-consistent dynamical modeling. The key issues are, stretched exponential character of dielectric relaxation, power-law power spectral density, and anomalous dependence of ac conduction coefficient on frequency. We propose a self-consistent model of dielectric relaxation, in which the relaxations are described by a stretched exponential decay function. Mathematically, our study refers to the expanding area of fractional calculus and we propose a systematic derivation of the fractional relaxation and fractional diffusion equations from the property of ac universality.
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