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Register a new userElectronic interlayer coupling in the LTT phase of La1.79Eu0.2Sr0.01CuO4
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Authors
M. Huecker
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The electronic interlayer transport of the lightly doped antiferromagnet La1.79Eu0.2Sr0.01CuO4 has been studied by means of magneto-resistance measurements. The central problem addressed concerns the differences between the electronic interlayer coupling in the tetragonal low-temperature (LTT) phase and the orthorhombic low-temperature (LTO) phase. The key observation is that the spin-flip induced drop in the c-axis magneto-resistance of the LTO phase, which is characteristic for pure La2-xSrxCuO4, dramatically decreases in the LTT phase. The results show that the transition from orthorhombic to tetragonal symmetry and from collinear to non-collinear antiferromagnetic spin structure eliminates the strain dependent anisotropic interlayer hopping as well as the concomitant spin-valve type transport channel. Implications for the stripe ordered LTT phase of La2-xBaxCuO4 are briefly discussed.
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The Cu spin magnetism in La2-x-yEuySrxCuO4 (x<=0.17; y<=0.2) has been studied by means of magnetization measurements up to 14 T. Our results clearly show that in the antiferromagnetic phase Dzyaloshinsky-Moriya (DM)superexchange causes Cu spin canting not only in the LTO phase but also in the LTLO and LTT phases. In La1.8Eu0.2CuO4 the canted DM-moment is about 50% larger than in pure La2CuO4 which we attribute to the larger octahedral tilt angle. We also find clear evidence that the size of the DM-moment does not change significantly at the structural transition at T_LT from LTO to LTLO and LTT. The most important change induced by the transition is a significant reduction of the magnetic coupling between the CuO2 planes. As a consequence, the spin-flip transition of the canted Cu spins which is observed in the LTO phase for magnetic field perpendicular to the CuO2 planes disappears in the LTT phase. The shape of the magnetization curves changes from the well known spin-flip type to a weak-ferromagnet type. However, no spontaneous weak ferromagnetism is observed even at very low temperatures, which seems to indicate that the interlayer decoupling in our samples is not perfect. Nonetheless, a small fraction (<15%) of the DM-moments can be remanently magnetized throughout the entire antiferromagnetically ordered LTT/LTLO phase, i.e. for T<T_LT and x<0.02. It appears that the remanent DM-moment is perpendicular to the CuO2 planes. For magnetic field parallel to the CuO2 planes we find that the critical field of the spin-flop transition decreases in the LTLO phase, which might indicate a competition between different in-plane anisotropies. To study the Cu spin magnetism in La2-x-yEuySrxCuO4, a careful analysis of the Van Vleck paramagnetism of the Eu3+ ions was performed.
Cuprate superconductors host a multitude of low-energy optical phonons. Using time- and angle-resolved photoemission spectroscopy, we study coherent phonons in Bi$_{2}$Sr$_{2}$Ca$_{0.92}$Y$_{0.08}$Cu$_{2}$O$_{8+delta}$. Sub-meV modulations of the electronic band structure are observed at frequencies of $3.94pm 0.01$ and $5.59pm 0.06$ THz. For the dominant mode at 3.94 THz, the amplitude of the band energy oscillation weakly increases as a function of momentum away from the node. Theoretical calculations allow identifying the observed modes as CuO$_{2}$-derived $A_{1g}$ phonons. The Bi- and Sr-derived $A_{1g}$ modes which dominate Raman spectra in the relevant frequency range are absent in our measurements. This highlights the mode-selectivity for phonons coupled to the near-Fermi-level electrons, which originate from CuO$_{2}$ planes and dictate thermodynamic properties.
We report an experimental determination of the dispersion of the soft phonon mode along [1,0,0] in uranium as a function of pressure. The energies of these phonons increase rapidly, with conventional behavior found by 20 GPa, as predicted by recent theory. New calculations demonstrate the strong pressure (and momentum) dependence of the electron-phonon coupling, whereas the Fermi-surface nesting is surprisingly independent of pressure. This allows a full understanding of the complex phase diagram of uranium, and the interplay between the charge-density wave and superconductivity.
The magnetic-field, temperature, and angular dependence of the interlayer magnetoresistance of two different quasi-two-dimensional (2D) organic superconductors is reported. For $kappa$-(BEDT-TTF)$_2$I$_3$ we find a well-resolved peak in the angle-dependent magnetoresistance at $Theta = 90^circ$ (field parallel to the layers). This clear-cut proof for the coherent nature of the interlayer transport is absent for $beta$-(BEDT-TTF)$_2$SF$_5$CH$_2$CF$_2$SO$_3$. This and the non-metallic behavior of the magnetoresistance suggest an incoherent quasiparticle motion for the latter 2D metal.
Cooperation and competition between the antiferromagnetic, d-wave superconducting and Mott-insulating states are explored for the two-dimensional Hubbard model including nearest and next-nearest-neighbor hoppings at zero temperature. Using the variational cluster approach with clusters of different shapes and sizes up to 10 sites, it is found that the doping-driven transition from a phase with microscopic coexistence of antiferromagnetism and superconductivity to a purely superconducting phase is discontinuous for strong interaction and accompanied by phase separation. At half-filling the system is in an antiferromagnetic Mott-insulating state with vanishing charge compressibility. Upon decreasing the interaction strength U below a certain critical value of roughly U=4 (in units of the nearest-neighbor hopping), however, the filling-dependent magnetic transition changes its character and becomes continuous. Phase separation or, more carefully, the tendency towards the formation of inhomogeneous states disappears. This critical value is in contrast to previous studies, where a much larger value was obtained. Moreover, we find that the system at half-filling undergoes the Mott transition from an insulator to a state with a finite charge compressibility at essentially the same value. The weakly correlated state at half-filling exhibits superconductivity microscopically admixed to the antiferromagnetic order. This scenario suggests a close relation between phase separation and the Mott-insulator physics.
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