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Register a new userDynamics of Photo-excited Spins in InSb Based Quantum Wells
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We report time resolved measurements of spin relaxation in doped and undoped InSb quantum wells using degenerate and two-color magneto-optical Kerr effect techniques. We observed that the photo-excited spin dynamics are strongly influenced by laser excitation fluence and the doping profile of the samples. In the low fluence regime, an oscillatory pattern was observed at low temperatures ($leq$ 77 K) in the samples with an asymmetric doping profile which might be attributed to the quasi-collision-free spin relaxation regime. Our measurements also suggest the influence of the barrier materials (Al$_{x}$In$_{1-x}$Sb) on the spin relaxation in these material systems.
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Irradiating a semiconductor with circularly polarized light creates spin-polarized charge carriers. If the material contains atoms with non-zero nuclear spin, they interact with the electron spins via the hyperfine coupling. Here, we consider GaAs/AlGaAs quantum wells, where the conduction-band electron spins interact with three different types of nuclear spins. The hyperfine interaction drives a transfer of spin polarization to the nuclear spins, which therefore acquire a polarization that is comparable to that of the electron spins. In this paper, we analyze the dynamics of the optical pumping process in the presence of an external magnetic field while irradiating a single quantum well with a circularly polarized laser. We measure the time dependence of the photoluminescence polarization to monitor the buildup of the nuclear spin polarization and thus the average hyperfine interaction acting on the electron spins. We present a simple model that adequately describes the dynamics of this process and is in good agreement with the experimental data.
We present molecular beam epitaxial grown single- and double-side $delta$-doped InAlSb/InSb quantum wells with varying distances down to 50 nm to the surface on GaSb metamorphic buffers. We analyze the surface morphology as well as the impact of the crystalline quality on the electron transport. Comparing growth on GaSb and GaAs substrates indicates that the structural integrity of our InSb quantum wells is solely determined by the growth conditions at the GaSb/InAlSb transition and the InAlSb barrier growth. The two-dimensional electron gas samples show high mobilities of up to 349 000 cm$^2$/Vs at cryogenic temperatures and 58 000 cm$^2$/Vs at room temperature. With the calculated Dingle ratio and a transport lifetime model, ionized impurities predominantly remote from the quantum well are identified as the dominant source of scattering events. The analysis of the well pronounced Shubnikov$-$de Haas oscillations reveals a high spin-orbit coupling with an effective $g$-factor of $-38.4$ in our samples. Along with the smooth surfaces and long mean free paths demonstrated, our InSb quantum wells are increasingly competitive for nanoscale implementations of Majorana mode devices.
We report on the observation of the cyclotron-resonance-assisted photon drag effect. Resonant photocurrent is detected in InSb/InAlSb quantum wells structures subjected to a static magnetic field and excited by terahertz radiation at oblique incidence. The developed theory based on Boltzmanns kinetic equation is in a good agreement with the experimental findings. We show that the resonant photocurrent originates from the transfer of photon momentum to free electrons drastically enhanced at cyclotron resonance.
We present a detailed analytical and numerical analysis of the nuclear spin dynamics in parabolic quantum wells. The shallow potential of parabolic quantum wells permits substantial modification of the electronic wave function in small electric fields. The nuclear spin relaxation via the hyperfine interaction depends on the electronic local density of states, therefore the local nuclear relaxation time depends sensitively on the electric field. For an inhomogeneous nuclear magnetization, such as generated by dynamic nuclear polarization, the total nuclear magnetization dynamics can similarly be altered. We examine this effect quantitatively and the effect of temperature, field, well thickness, and nuclear spin diffusion.
Organic-inorganic layered perovskites are two-dimensional quantum wells with layers of lead-halide octahedra stacked between organic ligand barriers. The combination of their dielectric confinement and ionic sublattice results in excitonic excitations with substantial binding energies that are strongly coupled to the surrounding soft, polar lattice. However, the ligand environment in layered perovskites can significantly alter their optical properties due to the complex dynamic disorder of soft perovskite lattice. Here, we observe the dynamic disorder through phonon dephasing lifetimes initiated by ultrafast photoexcitation employing high-resolution resonant impulsive stimulated Raman spectroscopy of a variety of ligand substitutions. We demonstrate that vibrational relaxation in layered perovskite formed from flexible alkyl-amines as organic barriers is fast and relatively independent of the lattice temperature. Relaxation in aromatic amine based layered perovskite is slower, though still fast relative to pure inorganic lead bromide lattices, with a rate that is temperature dependent. Using molecular dynamics simulations, we explain the fast rates of relaxation by quantifying the large anharmonic coupling of the optical modes with the ligand layers and rationalize the temperature independence due to their amorphous packing. This work provides a molecular and time-domain depiction of the relaxation of nascent optical excitations and opens opportunities to understand how they couple to the complex layered perovskite lattice, elucidating design principles for optoelectronic devices.
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