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New Stellar $(n,gamma)$ Cross Sections and The Karlsruhe Astrophysical Database of Nucleosynthesis in Stars

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 Added by Iris Dillmann
 Publication date 2008
  fields Physics
and research's language is English




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Since April 2005 a regularly updated stellar neutron cross section compilation is available online at http://nuclear-astrophysics.fzk.de/kadonis. This online-database is called the Karlsruhe Astrophysical Database of Nucleosynthesis in Stars project and is based on the previous Bao et al. compilation from the year 2000. The present version textsc{KADoNiS} v0.2 (January 2007) includes recommended cross sections for 280 isotopes between $^{1}$H and $^{210}$Po and 75 semi-empirical estimates for isotopes without experimental information. Concerning stellar $(n,gamma)$ cross sections of the 32 stable, proton-rich isotopes produced by the $p$ process experimental information is only available for 20 isotopes, but 9 of them have rather large uncertainties of $geq$9%. The first part of a systematic study of stellar $(n,gamma)$ cross sections of the $p$-process isotopes $^{74}$Se, $^{84}$Sr, $^{102}$Pd, $^{120}$Te, $^{130}$Ba, $^{132}$Ba, $^{156}$Dy, and $^{174}$Hf is presented. In another application textsc{KADoNiS} v0.2 was used for an modification of a reaction library of Basel university. With this modified library $p$-process network calculations were carried out and compared to previous results.



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The KADoNiS (Karlsruhe Astrophysical Database of Nucleosynthesis in Stars) project is an astrophysical online database for cross sections relevant for nucleosynthesis in the $s$ process and the $gamma$ process. The $s$-process database (www.kadonis.org) was started in 2005 and is presently facing its 4th update (KADoNiS v1.0). The $gamma$-process database (KADoNiS-p, www.kadonis.org/pprocess) was recently revised and re-launched in March 2013. Both databases are compilations for experimental cross sections with relevance to heavy ion nucleosynthesis. For the $s$ process recommended Maxwellian averaged cross sections for $kT$= 5-100~keV are given for more than 360 isotopes between $^{1}$H and $^{210}$Bi. For the $gamma$-process database all available experimental data from $(p,gamma), (p,n), (p,alpha), (alpha,gamma), (alpha,n)$, and $(alpha,p)$ reactions between $^{70}$Ge and $^{209}$Bi in or close to the respective Gamow window were collected and can be compared to theoretical predictions. The aim of both databases is a quick and user-friendly access to the available data in the astrophysically relevant energy regions.
The nucleosynthesis of elements beyond iron is dominated by the s and r processes. However, a small amount of stable isotopes on the proton-rich side cannot be made by neutron capture and are thought to be produced by photodisintegration reactions on existing seed nuclei in the so-called p process. So far most of the p-process reactions are not yet accessible by experimental techniques and have to be inferred from statistical Hauser-Feshbach model calculations. The parametrization of these models has to be constrained by measurements on stable proton-rich nuclei. A series of (n,$gamma$) activation measurements on p nuclei, related by detailed balance to the respective photodisintegrations, were carried out at the Karlsruhe Van de Graaff accelerator using the $^7$Li(p,n)$^7$Be source for simulating a Maxwellian neutron distribution of kT= 25 keV. We present here preliminary results of our extended measuring program in the mass range between A=74 and A=132, including first experimental (n,$gamma$) cross sections of $^{74}$Se, $^{84}$Sr, $^{120}$Te and $^{132}$Ba, and an improved value for $^{130}$Ba. In all cases we find perfect agreement with the recommended MACS predictions from the Bao et al. compilation.
Photoneutron cross sections were measured for $^{58}$Ni, $^{60}$Ni, $^{61}$Ni, and $^{64}$Ni at energies between the one-neutron and two-neutron thresholds using quasi-monochromatic $gamma$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. The new photoneutron data are used to extract the $gamma$-ray strength function above the neutron threshold complementing the information obtained by the Oslo method below the threshold. We discuss radiative neutron capture cross sections and the Maxwellian-averaged cross sections for Ni isotopes including $^{63}$Ni, a branching point nucleus along the weak s-process path. The cross sections are calculated with the experimentally constrained $gamma$-ray strength functions from the Hartree-Fock-Bogolyubov plus quasi-particle-random phase approximation based on the Gogny D1M interaction for both $E1$ and $M1$ components and supplemented with the $M1$ upbend.
The propagation of uncertainties in reaction cross sections and rates of neutron-, proton-, and alpha-induced reactions into the final isotopic abundances obtained in nucleosynthesis models is an important issue in studies of nucleosynthesis and Galactic Chemical Evolution. We developed a Monte Carlo method to allow large-scale postprocessing studies of the impact of nuclear uncertainties on nucleosynthesis. Temperature-dependent rate uncertainties combining realistic experimental and theoretical uncertainties are used. From detailed statistical analyses uncertainties in the final abundances are derived as probability density distributions. Furthermore, based on rate and abundance correlations an automated procedure identifies the most important reactions in complex flow patterns from superposition of many zones or tracers. The method so far was already applied to a number of nucleosynthesis processes. Here we focus on the production of p-nuclei in white dwarfs exploding as thermonuclear (type Ia) supernovae. We find generally small uncertainties in the final abundances despite of the dominance of theoretical nuclear uncertainties. A separate analysis of low- and high-density regions indicates that the total uncertainties are dominated by the high-density regions.
The $^{58}$Ni$(n,gamma)^{59}$Ni cross section was measured with a combination of the activation technique and accelerator mass spectrometry (AMS). The neutron activations were performed at the Karlsruhe 3.7 MV Van de Graaff accelerator using the quasi-stellar neutron spectrum at $kT=25$ keV produced by the $^7$Li($p,n$)$^7$Be reaction. The subsequent AMS measurements were carried out at the 14 MV tandem accelerator of the Maier-Leibnitz-Laboratory in Garching using the Gas-filled Analyzing Magnet System (GAMS). Three individual samples were measured, yielding a Maxwellian-averaged cross section at $kT=30$ keV of $langlesigmarangle_{30text{keV}}$= 30.4 (23)$^{syst}$(9)$^{stat}$ mbarn. This value is slightly lower than two recently published measurements using the time-of-flight (TOF) method, but agrees within the uncertainties. Our new results also resolve the large discrepancy between older TOF measurements and our previous value.
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