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(n,$gamma$) Cross Sections of Light p Nuclei -- Towards an Updated Database for the p Process

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 Added by Iris Dillmann
 Publication date 2008
  fields Physics
and research's language is English




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The nucleosynthesis of elements beyond iron is dominated by the s and r processes. However, a small amount of stable isotopes on the proton-rich side cannot be made by neutron capture and are thought to be produced by photodisintegration reactions on existing seed nuclei in the so-called p process. So far most of the p-process reactions are not yet accessible by experimental techniques and have to be inferred from statistical Hauser-Feshbach model calculations. The parametrization of these models has to be constrained by measurements on stable proton-rich nuclei. A series of (n,$gamma$) activation measurements on p nuclei, related by detailed balance to the respective photodisintegrations, were carried out at the Karlsruhe Van de Graaff accelerator using the $^7$Li(p,n)$^7$Be source for simulating a Maxwellian neutron distribution of kT= 25 keV. We present here preliminary results of our extended measuring program in the mass range between A=74 and A=132, including first experimental (n,$gamma$) cross sections of $^{74}$Se, $^{84}$Sr, $^{120}$Te and $^{132}$Ba, and an improved value for $^{130}$Ba. In all cases we find perfect agreement with the recommended MACS predictions from the Bao et al. compilation.

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High-statistics differential cross sections for the reactions gamma p -> p eta and gamma p -> p eta-prime have been measured using the CLAS at Jefferson Lab for center-of-mass energies from near threshold up to 2.84 GeV. The eta-prime results are the most precise to date and provide the largest energy and angular coverage. The eta measurements extend the energy range of the worlds large-angle results by approximately 300 MeV. These new data, in particular the eta-prime measurements, are likely to help constrain the analyses being performed to search for new baryon resonance states.
The total cross sections for the $^{152}$Gd(p,$gamma$)$^{153}$Tb and $^{152}$Gd(p,n)$^{152}$Tb reactions have been measured by the activation method at effective center-of-mass energies mbox{$3.47 leq E_mathrm{c.m.}^mathrm{eff}leq 7.94$ MeV} and mbox{$4.96 leq E_mathrm{c.m.}^mathrm{eff} leq 7.94$ MeV}, respectively. The targets were prepared by evaporation of 30.6% isotopically enriched $^{152}$Gd oxide on aluminum backing foils, and bombarded with proton beams provided by a cyclotron accelerator. The cross sections were deduced from the observed $gamma$-ray activity, which was detected off-line by a HPGe detector in a low background environment. The results are presented and compared with predictions of statistical model calculations. This comparison supports a modified optical proton+$^{152}$Gd potential suggested earlier.
Since April 2005 a regularly updated stellar neutron cross section compilation is available online at http://nuclear-astrophysics.fzk.de/kadonis. This online-database is called the Karlsruhe Astrophysical Database of Nucleosynthesis in Stars project and is based on the previous Bao et al. compilation from the year 2000. The present version textsc{KADoNiS} v0.2 (January 2007) includes recommended cross sections for 280 isotopes between $^{1}$H and $^{210}$Po and 75 semi-empirical estimates for isotopes without experimental information. Concerning stellar $(n,gamma)$ cross sections of the 32 stable, proton-rich isotopes produced by the $p$ process experimental information is only available for 20 isotopes, but 9 of them have rather large uncertainties of $geq$9%. The first part of a systematic study of stellar $(n,gamma)$ cross sections of the $p$-process isotopes $^{74}$Se, $^{84}$Sr, $^{102}$Pd, $^{120}$Te, $^{130}$Ba, $^{132}$Ba, $^{156}$Dy, and $^{174}$Hf is presented. In another application textsc{KADoNiS} v0.2 was used for an modification of a reaction library of Basel university. With this modified library $p$-process network calculations were carried out and compared to previous results.
With analyzing the solar system abundance, we have found two universal scaling laws concerning the p- and s-nuclei. They indicate that the gamma-process in supernova (SN) explosions is the most promising origin of the p-nuclei that has been discussed with many possible nuclear reactions and sites for about fifty years. In addition the scalings provide new concepts: an universality of the gamma-process and a new nuclear cosmochronometer. We have carried out gamma-process nucleosynthesis calculations for typical core-collapse SN explosion models and the results satisfy the observed scalings.
We have investigated the (n,gamma) cross sections of p-process isotopes with the activation technique. The measurements were carried out at the Karlsruhe Van de Graaff accelerator using the 7Li(p,n)7Be source for simulating a Maxwellian neutron distribution of kT = 25 keV. Stellar cross section measurements are reported for the light p-process isotopes 102Pd, 120Te, 130,132Ba, and 156Dy. In a following paper the cross sections of 168Yb, 180W, 184Os, 190Pt, and 196Hg will be discussed. The data are extrapolated to p-process energies by including information from evaluated nuclear data libraries. The results are compared to standard Hauser-Feshbach models frequently used in astrophysics.
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