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Optical spectra of the heavy fermion uniaxial ferromagnet UGe$_2$

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 Added by Violeta Guritanu
 Publication date 2008
  fields Physics
and research's language is English




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We report a detailed study of UGe$_{2}$ single crystals using infrared reflectivity and spectroscopic ellipsometry. The optical conductivity suggests the presence of a low frequency interband transition and a narrow free-carrier response with strong frequency dependence of the scattering rate and effective mass. We observe sharp changes in the low frequency mass and scattering rate below the upper ferromagnetic transition $T_C = 53 K$. The characteristic changes are exhibited most strongly at an energy scale of around 12 meV (100 cm$^{-1}$). They recover their unrenormalized value above $T_C$ and for $omega >$ 40 meV. In contrast no sign of an anomaly is seen at the lower transition temperature of unknown nature $T_x sim$ 30 K, observed in transport and thermodynamic experiments. In the ferromagnetic state we find signatures of a strong coupling to the longitudinal magnetic excitations that have been proposed to mediate unconventional superconductivity in this compound.



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We present thermoelectric power and resistivity measurements in the ferromagnet UGe$_2$ as a function of temperature and magnetic field. At low temperature, huge quantum oscillations are observed in the thermoelectric power as a function of the magnetic field applied along the $a$ axis. The frequencies of the extreme orbits are determined and an analysis of the cyclotron masses is performed following different theoretical approaches for quantum oscillations detected in the thermoelectric power. They are compared to those obtained by Shubnikov-de Haas experiments on the same crystal and previous de Haas-van Alphen experiments. The agreement of the different probes confirms thermoelectric power as an excellent probe to extract simultaneously both microscopic and macroscopic information on the Fermi-surface properties. Band-structure calculations of UGe$_2$ in the ferromagnetic state are compared to the experiment.
60 - D. Wulferding , H. Kim , I. Yang 2017
In search of novel, improved materials for magnetic data storage and spintronic devices, compounds that allow a tailoring of magnetic domain shapes and sizes are essential. Good candidates are materials with intrinsic anisotropies or competing interactions, as they are prone to host various domain phases that can be easily and precisely selected by external tuning parameters such as temperature and magnetic field. Here, we utilize vector magnetic fields to visualize directly the magnetic anisotropy in the uniaxial ferromagnet CeRu$_2$Ga$_2$B. We demonstrate a feasible control both globally and locally of domain shapes and sizes by the external field as well as a smooth transition from single stripe to bubble domains, which opens the door to future applications based on magnetic domain tailoring.
We report a comprehensive investigation of the lattice dynamics of URu$_2$Si$_2$ as a function of temperature using Raman scattering, optical conductivity and inelastic neutron scattering measurements as well as theoretical {it ab initio} calculations. The main effects on the optical phonon modes are related to Kondo physics. The B$_{1g}$ ($Gamma_3$ symmetry) phonon mode slightly softens below $sim$100~K, in connection with the previously reported softening of the elastic constant, $C_{11}-C_{12}$, of the same symmetry, both observations suggesting a B$_{1g}$ symmetry-breaking instability in the Kondo regime. Through optical conductivity, we detect clear signatures of strong electron-phonon coupling, with temperature dependent spectral weight and Fano line shape of some phonon modes. Surprisingly, the line shapes of two phonon modes, E$_u$(1) and A$_{2u}$(2), show opposite temperature dependencies. The A$_{2u}$(2) mode loses its Fano shape below 150 K, whereas the E$_u$(1) mode acquires it below 100~K, in the Kondo cross-over regime. This may point out to momentum-dependent Kondo physics. By inelastic neutron scattering measurements, we have drawn the full dispersion of the phonon modes between 300~K and 2~K. No remarkable temperature dependence has been obtained including through the hidden order transition. {it Ab initio} calculations with the spin-orbit coupling are in good agreement with the data except for a few low energy branches with propagation in the (a,b) plane.
The effect of uniaxial pressure (P_u) on the magnetic susceptibility (X), magnetization (M), and magnetoresistance (MR) of the heavy-fermion metamagnet CeRu2Si2 has been investigated. For the magnetic field along the tetragonal c axis, it is found that characteristic physical quantities, i.e., the temperature of the susceptibility maximum (T_max), the pagamagnetic Weiss temperature (Q_p), 1/X at 2 K, and the magnetic field of the metamagnetic anomaly (H_M), scale approximately linearly with P_u, indicating that all the quantities are related to the same energy scale, probably of the Kondo temperature. The increase (decrease) of the quantities for P_u || c axis (P_u || a axis) can be attributed to a decrease (increase) in the nearest Ce-Ru distance. Consistently in MR and X, we observed a sign that the anisotropic nature of the hybridization, which is believed to play an important role in the metamagnetic anomaly, can be controlled by applying the uniaxial pressure. PACS numbers: 75.20.Hr, 71.27.+a, 74.62.Fj
Physical properties of polycrystalline CeCrGe$_{3}$ and LaCrGe$_{3}$ have been investigated by x-ray absorption spectroscopy, magnetic susceptibility $chi(T)$, isothermal magnetization M(H), electrical resistivity $rho(T)$, specific heat C($T$) and thermoelectric power S($T$) measurements. These compounds are found to crystallize in the hexagonal perovskite structure (space group textit{P6$_{3}$/mmc}), as previously reported. The $rho(T)$, $chi(T)$ and C($T$) data confirm the bulk ferromagnetic ordering of itinerant Cr moments in LaCrGe$_{3}$ and CeCrGe$_{3}$ with $T_{C}$ = 90 K and 70 K respectively. In addition a weak anomaly is also observed near 3 K in the C($T$) data of CeCrGe$_{3}$. The T dependences of $rho$ and finite values of Sommerfeld coefficient $gamma$ obtained from the specific heat measurements confirm that both the compounds are of metallic character. Further, the $T$ dependence of $rho$ of CeCrGe$_{3}$ reflects a Kondo lattice behavior. An enhanced $gamma$ of 130 mJ/mol,K$^{2}$ together with the Kondo lattice behavior inferred from the $rho(T)$ establish CeCrGe$_{3}$ as a moderate heavy fermion compound with a quasi-particle mass renormalization factor of $sim$ 45.
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