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The electric quadrupole coupling constant of the ground state of 37K(3/2+, 1.22 s) in a tetragonal KH2PO4 single crystal was measured to be |eqQ/h| = 2.99 +- 0.07 MHz using the beta-ray detecting nuclear quadrupole resonance technique. The electric quadrupole moment of 37K was determined to be |Q(37K)| = 10.6 +- 0.4 efm2, where the known electric quadrupole coupling constant of stable 39K in the KH2PO4 crystal was used as a reference. The present experimental result is larger than that predicted by shell-model calculations in the sd or the sd and fp model spaces. A possible variation of effective charges was explored to explain the discrepancy.
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Ground-state electric quadrupole moment of 31Al (I =5/2+, T_1/2 = 644(25) ms) has been measured by means of the beta-NMR spectroscopy using a spin-polarized 31Al beam produced in the projectile fragmentation reaction. The obtained Q moment, |Q_exp(31Al)| = 112(32)emb, are in agreement with conventional shell model calculations within the sd valence space. Previous result on the magnetic moment also supports the validity of the sd model in this isotope, and thus it is concluded that 31Al is located outside of the island of inversion.
The electric quadrupole moment of the 33Al20 ground state, located at the border of the island of inversion, was obtained using continuous-beam beta-detected nuclear quadrupole resonance (beta-NQR). From the measured quadrupole coupling constant Q = 2.31(4) MHz in an alpha-Al2O3 crystal, a precise value for the electric quadrupole moment is extracted: Qs= 141(3) mb. A comparison with large-scale shell model calculations shows that 33Al has at least 50% intruder configurations in the ground state wave function, favoring the excitation of two neutrons across the N = 20 shell gap. 33Al therefore clearly marks the gradual transition north of the deformed Na and Mg nuclei towards the normal Z>14 isotopes.
he electric quadrupole coupling constant of the 31Al ground state is measured to be nu_Q = |eQV_{zz}/h| = 2196(21)kHz using two different beta-NMR (Nuclear Magnetic Resonance) techniques. For the first time, a direct comparison is made between the continuous rf technique and the adiabatic fast passage method. The obtained coupling constants of both methods are in excellent agreement with each other and a precise value for the quadrupole moment of 31Al has been deduced: |Q(31Al)| = 134.0(16) mb. Comparison of this value with large-scale shell-model calculations in the sd and sdpf valence spaces suggests that the 31Al ground state is dominated by normal sd-shell configurations with a possible small contribution of intruder states. The obtained value for |Q(31Al)| and a compilation of measured quadrupole moments of odd-Z even-N isotopes in comparison with shell-model calculations shows that the proton effective charge e_p=1.1 e provides a much better description of the nuclear properties in the sd-shell than the adopted value e_p=1.3 e.
The hyperfine splitting of the 5g -> 4f transitions in muonic 185,187-Re has been measured using high resolution HPGe detectors and compared to state-of-the-art atomic theoretical predictions. The spectroscopic quadrupole moment has been extracted using modern fitting procedures and compared to the values available in literature obtained from muonic X rays of natural rhenium. The extracted values of the nuclear spectroscopic quadrupole moment are 2.07(5) barn and 1.94(5) barn, respectively for 185-Re and 187-Re. This work is part of a larger effort at the Paul Scherrer Institut towards the measurement of the nuclear charge radii of radioactive elements.
The nuclear quadrupole moment of the I=3/2- excited nuclear state of 57Fe at 14.41 keV, important in Mossbauer spectroscopy, is determined from the large-scale nuclear shell-model calculations for 57Fe and also from the electronic ab initio and density functional theory calculations including solid state and electron correlation effects for the molecules Fe(CO)_5 and Fe(C_5 H_5)_2. Both independent methods yield very similar results. The recommended value is 0.16(1) eb. The NQM of the isomeric 10+ in 54Fe has also been calculated. The new value (0.5 eb), consistent with the perturbed angular distribution data, is by a factor of two larger than the currently recommended value.
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