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Register a new userObservation of Non-Exponential Orbital Electron Capture Decays of Hydrogen-Like $^{140}$Pr and $^{142}$Pm Ions
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We report on time-modulated two-body weak decays observed in the orbital electron capture of hydrogen-like $^{140}$Pr$^{59+}$ and $^{142}$Pm$^{60+}$ ions coasting in an ion storage ring. Using non-destructive single ion, time-resolved Schottky mass spectrometry we found that the expected exponential decay is modulated in time with a modulation period of about 7 seconds for both systems. Tentatively this observation is attributed to the coherent superposition of finite mass eigenstates of the electron neutrinos from the weak decay into a two-body final state.
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An experiment addressing electron capture (EC) decay of hydrogen-like $^{142}$Pm$^{60+}$ ions has been conducted at the experimental storage ring (ESR) at GSI. The decay appears to be purely exponential and no modulations were observed. Decay times for about 9000 individual EC decays have been measured by applying the single-ion decay spectroscopy method. Both visually and automatically analysed data can be described by a single exponential decay with decay constants of 0.0126(7) s$^{-1}$ for automatic analysis and 0.0141(7) s$^{-1}$ for manual analysis. If a modulation superimposed on the exponential decay curve is assumed, the best fit gives a modulation amplitude of merely 0.019(15), which is compatible with zero and by 4.9 standard deviations smaller than in the original observation which had an amplitude of 0.23(4).
We report on the first measurement of the $beta^+$- and orbital electron capture decay rates of $^{140}$Pr nuclei with the most simple electron configurations: bare nuclei, hydrogen-like and helium-like ions. The measured electron capture decay constant of hydrogen-like $^{140}$Pr$^{58+}$ ions is about 50% larger than that of helium-like $^{140}$Pr$^{57+}$ ions. Moreover, $^{140}$Pr ions with one bound electron decay faster than neutral $^{140}$Pr$^{0+}$ atoms with 59 electrons. To explain this peculiar observation one has to take into account the conservation of the total angular momentum, since only particular spin orientations of the nucleus and of the captured electron can contribute to the allowed decay.
The periodic time modulations, found recently in the two-body orbital electron-capture (EC) decay of both, hydrogen-like $^{140}$Pr$^{58+}$ and $^{142}$Pm$^{60+}$ ions, with periods near to 7s and amplitudes of about 20%, were re-investigated for the case of $^{142}$Pm$^{60+}$ by using a 245 MHz resonator cavity with a much improved sensitivity and time resolution. We observed that the exponential EC decay is modulated with a period $T = 7.11(11)$s, in accordance with a modulation period $T = 7.12(11)$ s as obtained from simultaneous observations with a capacitive pick-up, employed also in the previous experiments. The modulation amplitudes amount to $a_R = 0.107(24)$ and $a_P = 0.134(27)$ for the 245 MHz resonator and the capacitive pick-up, respectively. These new results corroborate for both detectors {it exactly} our previous findings of modulation periods near to 7s, though with {it distinctly smaller} amplitudes. Also the three-body $beta^+$ decays have been analyzed. For a supposed modulation period near to 7s we found an amplitude $a = 0.027(27)$, compatible with $a = 0$ and in agreement with the preliminary result $a = 0.030(30)$ of our previous experiment. These observations could point at weak interaction as origin of the observed 7s-modulation of the EC decay. Furthermore, the data suggest that interference terms occur in the two-body EC decay, although the neutrinos are not directly observed.
We have searched for time modulation of the electron capture decay probability of $^{142}$Pm in an attempt to confirm a recent claim from a group at the Gesellschaft f{u}r Schwerionenforschung (GSI). We produced $^{142}$Pm via the $^{124}$Sn($^{23}$Na, 5n)$^{142}$Pm reaction at the Berkeley 88-Inch Cyclotron with a bombardment time short compared to the reported modulation period. Isotope selection by the Berkeley Gas-filled Separator is followed by implantation and a long period of monitoring the $^{142}$Nd K$_{alpha}$ x-rays from the daughter. The decay time spectrum of the x-rays is well-described by a simple exponential and the measured half-life of 40.68(53) seconds is consistent with the accepted value. We observed no oscillatory modulation at the proposed frequency at a level 31 times smaller than that reported by Litvinov {it et al.} (Phys. Lett. B 664 (2008) 162; arXiv:0801.2079 [nucl-ex]). A literature search for previous experiments that might have been sensitive to the reported modulation uncovered another example in $^{142}$Eu electron-capture decay. A reanalysis of the published data shows no oscillatory behavior.
It is argued that orbital electron-capture decays of neutral $^{142}$Pm atoms implanted into the lattice of a solid (LBNL experiment) do not fulfil the constraints of true two-body beta decays, since momentum as well as energy of the final state are distributed among three objects, namely the electron neutrino, the recoiling daughter atom and the lattice phonons. To our understanding, this could be a reason for the non-observation of a periodic time modulation in the number of electron-capture decays of implanted neutral $^{142}$Pm atoms.
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