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Effects of strong correlations for 2D Bose-Einstein condensed dipolar excitons

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 Added by Yurii Lozovik
 Publication date 2007
  fields Physics
and research's language is English




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By doing quantum Monte Carlo ab initio simulations we show that dipolar excitons, which are now under experimental study, actually are strongly correlated systems. Strong correlations manifest in significant deviations of excitation spectra from the Bogoliubov one, large Bose condensate depletion, short-range order in the pair correlation function, and peak(s) in the structure factor.



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The Bose condensation of 2D dipolar excitons in quantum wells is numerically studied by the diffusion Monte Carlo simulation method. The correlation, microscopic, thermodynamic, and spectral characteristics are calculated. It is shown that, in structures of coupled quantum wells, in which low-temperature features of exciton luminescence have presently been observed, dipolar excitons form a strongly correlated system. Their Bose condensation can experimentally be achieved much easily than for ideal or weakly correlated excitons.
Correlations of luminescence intensity have been studied under Bose-Einstein condensation of dipolar excitons in the temperature range of 0.45-4.2 K. Photoexcited dipolar excitons were collected in a lateral trap in GaAs/AlGaAs Schottky-diode heterostructure with single wide (25 nm) quantum well under applied electric bias. Two-photon correlations were measured with the use of a classical Hanbury Brown - Twiss intensity interferometer (time resolution ~0.4 ns). Photon bunching has been observed near the Bose condensation threshold of dipolar excitons determined by the appearance of a narrow luminescence line of exciton condensate at optical pumping increase. The two-photon correlation function shows super-poissonian distribution at time scales of system coherence (<~1 ns). No photon bunching was observed at the excitation pumping appreciably below the condensation threshold. At excitation pumping increasing well above the threshold, when the narrow line of exciton condensate grows in the luminescence spectrum, the photon bunching is decreasing and finally vanishes - the two-photon correlator becomes poissonian reflecting the single-quantum-state origin of excitonic Bose condensate. Under the same conditions a first-order spatial correlator, measured by means of the luminescence interference from spatially separated condensate parts, remains significant. The discovered photon bunching is rather sensitive to temperature: it drops several times with temperature increase from 0.45 K up to 4.2 K. If assumed that the luminescence of dipolar excitons collected in the lateral trap reflects directly coherent properties of interacting exciton gas, the observed phenomenon of photon bunching nearby condensation threshold manifests phase transition in interacting exciton Bose gas.
We investigate the properties of quantized vortices in a dipolar Bose-Einstein condensed gas by means of a generalised Gross-Pitaevskii equation. The size of the vortex core hugely increases by increasing the weight of the dipolar interaction and approaching the transition to the supersolid phase. The critical angular velocity for the existence of an energetically stable vortex decreases in the supersolid, due to the reduced value of the density in the interdroplet region. The angular momentum per particle associated with the vortex line is shown to be smaller than $hbar$, reflecting the reduction of the global superfluidity. The real-time vortex nucleation in a rotating trap is shown to be triggered, as for a standard condensate, by the softening of the quadrupole mode. For large angular velocities, when the distance between vortices becomes comparable to the interdroplet distance, the vortices are arranged into a honeycomb structure, which coexists with the triangular geometry of the supersolid lattice and persists during the free expansion of the atomic cloud.
An exciton is an electron-hole pair bound by attractive Coulomb interaction. Short-lived excitons have been detected by a variety of experimental probes in numerous contexts. An excitonic insulator, a collective state of such excitons, has been more elusive. Here, thanks to Nernst measurements in pulsed magnetic fields, we show that in graphite there is a critical temperature (T = 9.2 K) and a critical magnetic field (B = 47 T) for Bose-Einstein condensation of excitons. At this critical field, hole and electron Landau sub-bands simultaneously cross the Fermi level and allow exciton formation. By quantifying the effective mass and the spatial separation of the excitons in the basal plane, we show that the degeneracy temperature of the excitonic fluid corresponds to this critical temperature. This identification would explain why the field-induced transition observed in graphite is not a universal feature of three-dimensional electron systems pushed beyond the quantum limit.
Bose-Einstein-condensed gases in external spatially random potentials are considered in the frame of a stochastic self-consistent mean-field approach. This method permits the treatment of the system properties for the whole range of the interaction strength, from zero to infinity, as well as for arbitrarily strong disorder. Besides a condensate and superfluid density, a glassy number density due to a spatially inhomogeneous component of the condensate occurs. For very weak interactions and sufficiently strong disorder, the superfluid fraction can become smaller than the condensate fraction, while at relatively strong interactions, the superfluid fraction is larger than the condensate fraction for any strength of disorder. The condensate and superfluid fractions, and the glassy fraction always coexist, being together either nonzero or zero. In the presence of disorder, the condensate fraction becomes a nonmonotonic function of the interaction strength, displaying an antidepletion effect caused by the competition between the stabilizing role of the atomic interaction and the destabilizing role of the disorder. With increasing disorder, the condensate and superfluid fractions jump to zero at a critical value of the disorder parameter by a first-order phase transition.
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