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Register a new userQuantum Spin Excitations through the metal-to-insulator crossover in $Y Ba_2 Cu_3 O_{6+y}$
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We use inelastic neutron scattering to study the temperature dependence of the spin excitations of a detwinned superconducting YBa$_2$Cu$_3$O$_{6.45}$ ($T_c=48$ K). In contrast to earlier work on YBa$_2$Cu$_3$O$_{6.5}$ ($T_c=58$ K), where the prominent features in the magnetic spectra consist of a sharp collective magnetic excitation termed ``resonance and a large ($hbaromegaapprox 15$ meV) superconducting spin gap, we find that the spin excitations in YBa$_2$Cu$_3$O$_{6.45}$ are gapless and have a much broader resonance. Our detailed mapping of magnetic scattering along the $a^ast$/$b^ast$-axis directions at different energies reveals that spin excitations are unisotropic and consistent with the ``hourglass-like dispersion along the $a^ast$-axis direction near the resonance, but they are isotropic at lower energies. Since a fundamental change in the low-temperature normal state of YBa$_2$Cu$_3$O$_{6+y}$ when superconductivity is suppressed takes place at $ysim0.5$ with a metal-to-insulator crossover (MIC), where the ground state transforms from a metallic to an insulating-like phase, our results suggest a clear connection between the large change in spin excitations and the MIC. The resonance therefore is a fundamental feature of metallic ground state superconductors and a consequence of high-$T_c$ superconductivity.
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Short-range lattice superstructures have been studied with high-energy x-ray diffuse scattering in underdoped, optimally doped, and overdoped $rm (Y,Ca)Ba_2 Cu_3 O_{6+x}$. A new four-unit-cell superstructure was observed in compounds with $xsim 0.95$. Its temperature, doping, and material dependence was used to attribute its origin to short-range oxygen vacancy ordering, rather than electronic instabilities in the $rm CuO_2$ layers. No significant diffuse scattering is observed in YBa$_2$Cu$_4$O$_{8}$. The oxygen superstructures must be taken into account when interpreting spectral anomalies in $rm (Y,Ca)Ba_2 Cu_3 O_{6+x}$.
The far-infrared dielectric response of superlattices (SL) composed of superconducting YBa$_{2}$Cu$_{3}$O$_{7}$ (YBCO) and ferromagnetic La$_{0.67}$% Ca$_{0.33}$MnO$_{3}$ (LCMO) has been investigated by ellipsometry. A drastic decrease of the free carrier response is observed which involves an unusually large length scale of d$^{crit}approx $20 nm in YBCO and d$^{crit}approx $10 nm in LCMO. A corresponding suppression of metallicity is not observed in SLs where LCMO is replaced by the paramagnetic metal LaNiO$_{3}$. Our data suggest that either a long range charge transfer from the YBCO to the LCMO layers or alternatively a strong coupling of the charge carriers to the different and competitive kind of magnetic correlations in the LCMO and YBCO layers are at the heart of the observed metal/insulator transition. The low free carrier response observed in the far-infrared dielectric response of the magnetic superconductor RuSr$_{2}$GdCu$_{2}$O$_{8}$ is possibly related to this effect.
We report on an infrared study of carrier dynamics within the CuO$_{2}$ planes in heavily underdoped detwinned single crystals of YBa$_{2}$Cu$_{3}$O$% _{y}$. In an effort to reveal the electronic structure near the onset of superconductivity, we investigate the strong anisotropy of the electromagnetic response due to an enhancement of the scattering rate along the a-axis. We propose that the origin of this anisotropy is related to a modulation of the electron density within the CuO$_{2}$ planes.
The irreversible magnetization of the layered high-T_{c} superconductor Bi_{2+x}Sr_{2-(x+y)}Cu_{1+y}O_{6 +- delta} (Bi-2201) has been measured by means of a capacitive torquemeter up to B=28 T and down to T=60 mK. No magnetization jumps, peak effects or crossovers between different pinning mechanisms appear to be present. The deduced irreversibility field B_{irr} can not be described by the law B_{irr}(T)=B_{irr}(0)(1-T/T_{c})^n based on flux creep, but an excellent agreement is found with the analytical form of the melting line of the flux lattice as calculated from the Lindemann criterion. The behavior of B_{irr}(T) obtained here is very similar to the resistive critical field of a Bi-2201 thin film, suggesting that magnetoresistive experiments are likely to be strongly influenced by flux lattice melting.
Superconductivity in cuprates peaks in the doping regime between a metal at high p and an insulator at low p. Understanding how the material evolves from metal to insulator is a fundamental and open question. Early studies in high magnetic fields revealed that below some critical doping an insulator-like upturn appears in the resistivity of cuprates at low temperature, but its origin has remained a puzzle. Here we propose that this metal-to-insulator crossover is due to a drop in carrier density n associated with the onset of the pseudogap phase at a critical doping p*. We use high-field resistivity measurements on LSCO to show that the upturns are quantitatively consistent with a drop from n=1+p above p* to n=p below p*, in agreement with high-field Hall data in YBCO. We demonstrate how previously reported upturns in the resistivity of LSCO, YBCO and Nd-LSCO are explained by the same universal mechanism: a drop in carrier density by 1.0 hole per Cu atom.
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