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Register a new userBlackbody radiation shift in a 43Ca+ ion optical frequency standard
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Motivated by the prospect of an optical frequency standard based on 43Ca+, we calculate the blackbody radiation (BBR) shift of the 4s_1/2-3d_5/2 clock transition, which is a major component of the uncertainty budget. The calculations are based on the relativistic all-order single-double method where all single and double excitations of the Dirac-Fock wave function are included to all orders of perturbation theory. Additional calculations are conducted for the dominant contributions in order to evaluate some omitted high-order corrections and estimate the uncertainties of the final results. The BBR shift obtained for this transition is 0.38(1) Hz. The tensor polarizability of the 3d_5/2 level is also calculated and its uncertainty is evaluated as well. Our results are compared with other calculations.
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We measure the dynamic differential scalar polarizabilities at 10.6 $mu$m for two candidate clock transitions in $^{176}mathrm{Lu}^+$. The fractional black body radiation (BBR) shifts at 300 K for the $^1S_0 leftrightarrow {^3D_1}$ and $^1S_0 leftrightarrow {^3D_2}$ transitions are evaluated to be $-1.36,(9) times 10^{-18}$ and $2.70 ,(21) times10^{-17}$, respectively. The former is the lowest of any established optical atomic clock.
We evaluated the static and dynamic polarizabilities of the 5s^2 ^1S_0 and 5s5p ^3P_0^o states of Sr using the high-precision relativistic configuration interaction + all-order method. Our calculation explains the discrepancy between the recent experimental 5s^2 ^1S_0 - 5s5p ^3P_0^o dc Stark shift measurement Delta alpha = 247.374(7) a.u. [Middelmann et. al, arXiv:1208.2848 (2012)] and the earlier theoretical result of 261(4) a.u. [Porsev and Derevianko, Phys. Rev. A 74, 020502R (2006)]. Our present value of 247.5 a.u. is in excellent agreement with the experimental result. We also evaluated the dynamic correction to the BBR shift with 1 % uncertainty; -0.1492(16) Hz. The dynamic correction to the BBR shift is unusually large in the case of Sr (7 %) and it enters significantly into the uncertainty budget of the Sr optical lattice clock. We suggest future experiments that could further reduce the present uncertainties.
A calculation of the blackbody radiation shift of the B$^+$ clock transition is performed. The polarizabilities of the B$^+$ $2s^2$ $^1$S$^e$, $2s2p$ $^1$P$^o$, and $2s2p$ $^3$P$^o$ states are computed using the configuration interaction method with an underlying semi-empirical core potential. The recommended dipole polarizabilities are 9.64(3) $a_0^3$, 7.78(3) $a_0^3$ and 16.55(5) $a_0^3$ respectively. The derived frequency shift for the $2s^2$ $^1$S$^e$ $to$ $2s2p$ $^3$P$^o_0$ transition at 300 K is 0.0160(5) Hz. The dipole polarizabilities agree with an earlier relativistic calculation (Safronova {em et al.} Phys. Rev. Lett. {bf 107} 143006 (2011)) to better than 0.2%. Quadrupole and octupole polarizabilities and non-adiabatic multipole polarizabilities are also reported.
Collisions with background gas can perturb the transition frequency of trapped ions in an optical atomic clock. We develop a non-perturbative framework based on a quantum channel description of the scattering process, and use it to derive a master equation which leads to a simple analytic expression for the collisional frequency shift. As a demonstration of our method, we calculate the frequency shift of the Sr$^+$ optical atomic clock transition due to elastic collisions with helium.
Black-body radiation (BBR) shifts of $^3!P_0-^1!S_0$ clock transition in divalent atoms Cd and Zn are evaluated using accurate relativistic many-body techniques of atomic structure. Static polarizabilities of the clock levels and relevant electric-dipole matrix elements are computed. We also present a comparative overview of the BBR shifts in optical clocks based on neutral divalent atoms trapped in optical lattices.
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