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Scattering mechanisms and Boltzmann transport in graphene

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 Added by Shaffique Adam
 Publication date 2007
  fields Physics
and research's language is English




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Different scattering mechanisms in graphene are explored and conductivity is calculated within the Boltzmann transport theory. We provide results for short-range scattering using the Random Phase Approximation for electron screening, as well as analytical expressions for the dependence of conductivity on the dielectric constant of the substrate. We further examine the effect of ripples on the transport using a surface roughness model developed for semiconductor heterostructures. We find that close to the Dirac point, sigma sim n^beta, where beta=1,0,-2 for Coulomb, short-range and surface roughness respectively; implying that Coulomb scattering dominates over both short-range and surface roughness scattering at low density.



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A Drude-Boltzmann theory is used to calculate the transport properties of bilayer graphene. We find that for typical carrier densities accessible in graphene experiments, the dominant scattering mechanism is overscreened Coulomb impurities that behave like short-range scatterers. We anticipate that the conductivity $sigma(n)$ is linear in $n$ at high density and has a plateau at low density corresponding to a residual density of $n^* = sqrt{n_{rm imp} {tilde n}}$, where ${tilde n}$ is a constant which we estimate using a self-consistent Thomas-Fermi screening approximation to be ${tilde n} approx 0.01 ~q_{rm TF}^2 approx 140 times 10^{10} {rm cm}^{-2}$. Analytic results are derived for the conductivity as a function of the charged impurity density. We also comment on the temperature dependence of the bilayer conductivity.
Using the semiclassical quantum Boltzmann equation (QBE), we numerically calculate the DC transport properties of bilayer graphene near charge neutrality. We find, in contrast to prior discussions, that phonon scattering is crucial even at temperatures below 40K. Nonetheless, electron-electron scattering still dominates over phonon collisions allowing a hydrodynamic approach. We introduce a simple two-fluid hydrodynamic model of electrons and holes interacting via Coulomb drag and compare our results to the full QBE calculation. We show that the two-fluid model produces quantitatively accurate results for conductivity, thermopower, and thermal conductivity.
We compare a fully quantum mechanical numerical calculation of the conductivity of graphene to the semiclassical Boltzmann theory. Considering a disorder potential that is smooth on the scale of the lattice spacing, we find quantitative agreement between the two approaches away from the Dirac point. At the Dirac point the two theories are incompatible at weak disorder, although they may be compatible for strong disorder. Our numerical calculations provide a quantitative description of the full crossover between the quantum and semiclassical graphene transport regimes.
214 - Hengyi Xu , Thomas Heinzel 2012
The conductivity of armchair graphene nanoribbons in the presence of short-range impurities and edge roughness is studied theoretically using the Boltzmann transport equation for quasi-one-dimensional systems. As the number of occupied subbands increases, the conductivity due to short-range impurities converges towards the two-dimensional case. Calculations of the magnetoconductivity confirm the edge-roughness-induced dips at cyclotron radii close to the ribbon width suggested by the recent quantum simulations.
243 - Hengyi Xu , T. Heinzel , 2011
We derive analytical expressions for the conductivity of bilayer graphene (BLG) using the Boltzmann approach within the the Born approximation for a model of Gaussian disorders describing both short- and long-range impurity scattering. The range of validity of the Born approximation is established by comparing the analytical results to exact tight-binding numerical calculations. A comparison of the obtained density dependencies of the conductivity with experimental data shows that the BLG samples investigated experimentally so far are in the quantum scattering regime where the Fermi wavelength exceeds the effective impurity range. In this regime both short- and long-range scattering lead to the same linear density dependence of the conductivity. Our calculations imply that bilayer and single layer graphene have the same scattering mechanisms. We also provide an upper limit for the effective, density dependent spatial extension of the scatterers present in the experiments.
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