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Register a new userNodal/Antinodal Dichotomy and the Two Gaps of a Superconducting Doped Mott Insulator
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We study the superconducting state of the hole-doped two-dimensional Hubbard model using Cellular Dynamical Mean Field Theory, with the Lanczos method as impurity solver. In the under-doped regime, we find a natural decomposition of the one-particle (photoemission) energy-gap into two components. The gap in the nodal regions, stemming from the anomalous self-energy, decreases with decreasing doping. The antinodal gap has an additional contribution from the normal component of the self-energy, inherited from the normal-state pseudogap, and it increases as the Mott insulating phase is approached.
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We introduce a valence-bond dynamical mean-field theory of doped Mott insulators. It is based on a minimal cluster of two orbitals, each associated with a different region of momentum space and hybridized to a self-consistent bath. The low-doping regime is characterized by singlet formation and the suppression of quasiparticles in the antinodal regions, leading to the formation of Fermi arcs. This is described in terms of an orbital-selective transition in reciprocal space. The calculated tunneling and photoemission spectra are consistent with the phenomenology of the normal state of cuprates. We derive a low-energy description of these effects using a generalization of the slave-boson method.
Recent angle-resolved photoemission electron spectroscopy (ARPES) experiments demonstrate that the momentum dependence of the spectral gap in underdoped cuprates does not follow a pure $d$-wave form [H. Anzai et a., Nat. Comm. {bf 4}, 1815 (2013)]. This deviation is highly controversial. It has often been interpretated as a proof of the non-superconducting origin of the antinodal gap in the underdoped regime. In this article, we show that the measured angular dependence of the spectral gap can be explained by the basic nature of pairs in high-T$_c$ cuprates. Hole pairs, or {it pairons}, form as a result of the local antiferromagnetic environment on the scale $xi_{AF}$, the magnetic coherence length. The spatial extension of the pairon wavefunction beyond first nearest neighbours gives rise to the anomalous angular dependence of the gap, in quantitative agreement with experiments. This simple interpretation strongly indicates a common origin of the nodal and antinodal gaps.
Detailed understanding of the role of single dopant atoms in host materials has been crucial for the continuing miniaturization in the semiconductor industry as local charging and trapping of electrons can completely change the behaviour of a device. Similarly, as dopants can turn a Mott insulator into a high temperature superconductor, their electronic behaviour at the atomic scale is of much interest. Due to limited time resolution of conventional scanning tunnelling microscopes, most atomic scale studies in these systems focussed on the time averaged effect of dopants on the electronic structure. Here, by using atomic scale shot-noise measurements in the doped Mott insulator Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$, we visualize sub-nanometer sized objects where remarkable dynamics leads to an enhancement of the tunnelling current noise by at least an order of magnitude. From the position, current and energy dependence we argue that these defects are oxygen dopant atoms that were unaccounted for in previous scanning probe studies, whose local environment leads to charge dynamics that strongly affect the tunnelling mechanism. The unconventional behaviour of these dopants opens up the possibility to dynamically control doping at the atomic scale, enabling the direct visualization of the effect of local charging on e.g. high T$_{text{c}}$ superconductivity.
How a Mott insulator develops into a weakly coupled metal upon doping is a central question to understanding various emergent correlated phenomena. To analyze this evolution and its connection to the high-$T_c$ cuprates, we study the single-particle spectrum for the doped Hubbard model using cluster perturbation theory on superclusters. Starting from extremely low doping, we identify a heavily renormalized quasiparticle dispersion that immediately develops across the Fermi level, and a weakening polaronic side band at higher binding energy. The quasiparticle spectral weight roughly grows at twice the rate of doping in the low doping regime, but this rate is halved at optimal doping. In the heavily doped regime, we find both strong electron-hole asymmetry and a persistent presence of Mott spectral features. Finally, we discuss the applicability of the single-band Hubbard model to describe the evolution of nodal spectra measured by angle-resolved photoemission spectroscopy (ARPES) on the single-layer cuprate La$_{2-x}$Sr$_x$CuO$_4$ ($0 le x le 0.15$). This work benchmarks the predictive power of the Hubbard model for electronic properties of high-$T_c$ cuprates.
Because the cuprate superconductors are doped Mott insulators, it would be advantageous to solve even a toy model that exhibits both Mottness and superconductivity. We consider the Hatsugai-Kohmoto model, an exactly solvable system that is a prototypical Mott insulator above a critical interaction strength at half filling. Upon doping or reducing the interaction strength, our exact calculations show that the system becomes a non-Fermi liquid metal with a superconducting instability. In the presence of a weak pairing interaction, the instability produces a thermal transition to a superconducting phase, which is distinct from the BCS state, as evidenced by a gap-to-transition temperature ratio exceeding the universal BCS limit. The elementary excitations of this superconductor are not Bogoliubov quasiparticles but rather superpositions of doublons and holons, composite excitations signaling that the superconducting ground state of the doped Mott insulator inherits the non-Fermi liquid character of the normal state. An unexpected feature of this model is that it exhibits a superconductivity-induced transfer of spectral weight from high to low energies as seen in the cuprates as well as a suppression of the superfluid density relative to that in BCS theory.
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