Magnetoelastic study on the frustrated quasi-one-dimensional spin-1/2 magnet LiCuVO$_4$


الملخص بالإنكليزية

We investigated the magnetoelastic properties of the quasi-one-dimensional spin-1/2 frustrated magnet LiCuVO$_4$. Longitudinal-magnetostriction experiments were performed at 1.5 K in high magnetic fields of up to 60 T applied along the $b$ axis, i.e., the spin-chain direction. The magnetostriction data qualitatively resemble the magnetization results, and saturate at $H_{text{sat}} approx 54$ T, with a relative change in sample length of $Delta L/L approx 1.8times10^{-4}$. Remarkably, both the magnetostriction and the magnetization evolve gradually between $H_{text{c3}} approx 48$ T and $H_{text{sat}}$, indicating that the two quantities consistently detect the spin-nematic phase just below the saturation. Numerical analyses for a weakly coupled spin-chain model reveal that the observed magnetostriction can overall be understood within an exchange-striction mechanism. Small deviations found may indicate nontrivial changes in local correlations associated with the field-induced phase transitions.

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