We present firstly the equation of motion for the test scalar particle coupling to the Chern-Simons invariant in Kerr black hole spacetime by the short-wave approximation. We have analyzed the dynamical behaviors of the test coupled particles by applying techniques including Poincare sections, fast Lyapunov exponent indicator, bifurcation diagram and basins of attraction. It is shown that there exists chaotic phenomenon in the motion of scalar particle interacted with the Chern-Simons invariant in a Kerr black hole spacetime. With the increase of the coupling strength, the motion of the coupled particles for the chosen parameters first undergoes a series of transitions betweens chaotic motion and regular motion and then falls into horizon or escapes to spatial infinity. Thus, the coupling between scalar particle and Chern-Simons invariant yields the richer dynamical behavior of scalar particle in a Kerr black hole spacetime.
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