Deterministically aperiodic sequences are an intermediary between periodic sequences and completely random sequences. Materials which are translationally periodic have Bloch-like extended states, while random media exhibit Anderson localisation. Materials constructed on the basis of deterministic aperiodic sequences such as Fibonacci, Thue-Morse, and Rudin-Shapiro exhibit different properties, which can be related to their spectrum. Here, by investigating the dynamics of discrete-time quantum walks using different aperiodic sequences of coin operations in position space and time we establish the role of the diffraction spectra in characterizing the spreading of the wavepacket.