We firstly demonstrate physically-prepared compliant PVA hydrogel electrodes as a promising supplement in dielectric elastomer actuators. They are capable of conducting high voltages over 5 kV without electrolysis by an electrical double layer effect. The hydrogel electrodes adhere tightly to the dielectric layer, which ensures its structural stability during actuation. All-polymeric actuators fabricated by these electrodes exhibited excellent consecutive working performance over 2960 cycles. The actuation was influenced by applied voltage, ramp rate, electrode elastic modulus and moisture content. A maximum areal strain over 78% was achieved. Tunable transparency, good biocompatibility, long lifetime, low cost and facile fabrication make PVA hydrogel electrode another promising candidate in the fields of sensors, artificial muscles and optical applications.
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