We observed quantum reflection of ultracold atoms from the attractive potential of a solid surface. Extremely dilute Bose-Einstein condensates of ^{23}Na, with peak density 10^{11}-10^{12}atoms/cm^3, confined in a weak gravito-magnetic trap were normally incident on a silicon surface. Reflection probabilities of up to 20 % were observed for incident velocities of 1-8 mm/s. The velocity dependence agrees qualitatively with the prediction for quantum reflection from the attractive Casimir-Polder potential. Atoms confined in a harmonic trap divided in half by a solid surface exhibited extended lifetime due to quantum reflection from the surface, implying a reflection probability above 50 %.
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