Crossover and Coexistence of Quasiparticle Excitations in the Fractional Quantum Hall Regime at $ u leq 1/3$

New low-lying excitations are observed by inelastic light scattering at filling factors $ u=p/(phi p pm 1)$ of the fractional quantum Hall regime with $phi=4$. Coexisting with these modes throughout the range $ u leq 1/3$ are $phi=2$ excitations seen at 1/3. Both $phi=2$ and $phi=4$ excitations have distinct behaviors with temperature and filling factor. The abrupt first appearance of the new modes in the low energy excitation spectrum at $ u lesssim 1/3$ suggests a marked change in the quantum ground state on crossing the $phi=2 to phi=4$ boundary at $ u = 1/3$.