We implement and investigate a method for measuring departures from scale-invariance, both scale-dependent as well as scale-free, in the primordial power spectrum of density perturbations using cosmic microwave background (CMB) C_l data and a principal component analysis technique. The primordial power spectrum is decomposed into a dominant scale-invariant Gaussian adiabatic component plus a series of orthonormal modes whose detailed form only depends the noise model for a particular CMB experiment. However, in general these modes are localised across wavenumbers with 0.01 < k < 0.2 Mpc^-1, displaying rapid oscillations on scales corresponding the acoustic peaks where the sensitivity to primordial power spectrum is greatest. The performance of this method is assessed using simulated data for the Planck satellite, and the full cosmological plus power spectrum parameter space is integrated out using Markov Chain Monte Carlo. As a proof of concept we apply this data compression technique to the current CMB data from WMAP, ACBAR, CBI and VSA. We find no evidence for the breaking of scale-invariance from measurements of four PCA mode amplitudes, which is translated to a constraint on the scalar spectral index n_S(k_0=0.04 Mpc^-1)=0.94+-0.04 in accordance with WMAP studies.
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